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Influence of catastrophes and hidden dynamical symmetries on ultrafast backscattered photoelectrons

Rook, T; Rodriguez, L Cruz; Figueira de Morisson Faria, C; (2024) Influence of catastrophes and hidden dynamical symmetries on ultrafast backscattered photoelectrons. Physical Review Research , 6 (2) , Article 023329. 10.1103/PhysRevResearch.6.023329. Green open access

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Abstract

We discuss the effect of using potentials with a Coulomb tail and different degrees of softening in photoelectron momentum distributions (PMDs) using the recently implemented hybrid forward-boundary CQSFA (H-CQSFA). We show that introducing a softening in the Coulomb interaction influences the ridges observed in the PMDs associated with backscattered electron trajectories. In the limit of a hard-core Coulomb interaction, the rescattering ridges close along the polarization axis, while for a soft-core potential, they are interrupted at ridge-specific angles. We analyze the momentum mapping of the different orbits leading to the ridges. For the hard-core potential, there exist two types of saddle-point solutions that coalesce at the ridge. By increasing the softening, we show that two additional solutions emerge as the result of breaking a hidden dynamical symmetry associated exclusively with the Coulomb potential. Further signatures of this symmetry breaking are encountered in subsets of momentum-space trajectories. Finally, we use scattering theory to show how the softening affects the maximal scattering angle and provide estimates that agree with our observations from the CQSFA. This implies that, in the presence of residual binding potentials in the electron's continuum propagation, the distinction between purely kinematic and dynamic caustics becomes blurred.

Type: Article
Title: Influence of catastrophes and hidden dynamical symmetries on ultrafast backscattered photoelectrons
Open access status: An open access version is available from UCL Discovery
DOI: 10.1103/PhysRevResearch.6.023329
Publisher version: https://doi.org/10.1103/physrevresearch.6.023329
Language: English
Additional information: Published by the American Physical Society under the terms of the Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article’s title, journal citation, and DOI.
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences > Dept of Physics and Astronomy
URI: https://discovery.ucl.ac.uk/id/eprint/10218851
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