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Magnetic structures of PrMn_{7}O_{12}: Intersublattice magnetoelastic coupling and incommensurate spin canting

Behr, D; Liu, R; Yamaura, K; Belik, AA; Khalyavin, DD; Johnson, RD; (2024) Magnetic structures of PrMn_{7}O_{12}: Intersublattice magnetoelastic coupling and incommensurate spin canting. Physical Review B , 110 (13) , Article 134426. 10.1103/PhysRevB.110.134426. Green open access

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Abstract

We report on the magnetic structures of PrMn7O12, resolving both a high-temperature structure in common with the other R3+Mn7O12 systems and an additional low-temperature phase characterized by a superposed incommensurate (ICM) spin canting. A phenomenological model is developed to account for large magnetoelastic coupling immediately below the Curie temperature, demonstrating that A′B exchange is primarily responsible for the ferrimagnetic structures observed across the R3+Mn7O12 family. Finally, an analytical mean-field minimal model is presented that successfully accounts for all magnetic structures observed in this family of materials, including the canted commensurate and ICM ground states.

Type: Article
Title: Magnetic structures of PrMn_{7}O_{12}: Intersublattice magnetoelastic coupling and incommensurate spin canting
Open access status: An open access version is available from UCL Discovery
DOI: 10.1103/PhysRevB.110.134426
Publisher version: http://dx.doi.org/10.1103/physrevb.110.134426
Language: English
Additional information: © 2024 American Physical Society. Published by the American Physical Society under the terms of the Creative Commons Attribution 4.0 International license (https://creativecommons.org/licenses/by/4.0/).
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences > Dept of Physics and Astronomy
URI: https://discovery.ucl.ac.uk/id/eprint/10201108
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