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Harmony of nanosystems: Graphitic carbon nitride/carbon nanomaterial hybrid architectures for energy storage in supercapacitors and batteries

Haruna, A; Dönmez, KB; Hooshmand, S; Avcı, E; Qamar, M; Zaidi, SA; Shahzad, F; ... Bayazıt, MK; + view all (2024) Harmony of nanosystems: Graphitic carbon nitride/carbon nanomaterial hybrid architectures for energy storage in supercapacitors and batteries. Carbon , 226 , Article 119177. 10.1016/j.carbon.2024.119177.

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Abstract

Developing high-performing and scalable electrode materials for supercapacitors and batteries has been of tremendous interest for the world's forthcoming clean and renewable energy transition. As a versatile material, Two-dimensional graphitic carbon nitride (g-CN) has been utilized in electrochemical energy storage (EES) applications due to its nitrogen-rich adsorption sites, cost-effective production, and tunable electronic structure. The electrochemical performance of pristine g-CN has been boosted by forming hybrid architectures with highly conductive carbon-based materials, such as graphene, reduced graphene oxide, carbon nanofibers, carbon nanotubes, and beyond (e.g., MXene). Using such heterogeneous compositions for EES applications has significantly increased in recent years. This study reviews the g-CN/carbon nanomaterial (CNM) hybrids, considering the dimensionality in nanomaterials, and underscores the influence of the material's dimensionality and the synthesis/fabrication routes. The effect of structural and physicochemical changes on the electrode's electrochemical performance after hybridization is presented comparatively. Besides, the comprehensive review outlines challenges and future improvements in g-CN/CNM hybrid materials for outstanding developments in energy storage systems

Type: Article
Title: Harmony of nanosystems: Graphitic carbon nitride/carbon nanomaterial hybrid architectures for energy storage in supercapacitors and batteries
DOI: 10.1016/j.carbon.2024.119177
Publisher version: http://dx.doi.org/10.1016/j.carbon.2024.119177
Language: English
Additional information: This version is the author accepted manuscript. For information on re-use, please refer to the publisher’s terms and conditions.
Keywords: Graphitic carbon nitride, Carbon nanomaterials, Hybrid electrodes, Supercapacitors, Batteries
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science > Dept of Chemical Engineering
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences > Dept of Physics and Astronomy
URI: https://discovery.ucl.ac.uk/id/eprint/10192968
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