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Fabrication and characterization of coated ceramic membranes from natural sources for water treatment applications

Alsubei, Mohammed D; Reid, Barry; Aljlil, Saad A; Coppens, Marc-Olivier; Campos, Luiza C; (2024) Fabrication and characterization of coated ceramic membranes from natural sources for water treatment applications. Journal of Membrane Science , 690 , Article 122226. 10.1016/j.memsci.2023.122226. (In press). Green open access

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Abstract

This study aimed to fabricate ceramic membranes for water treatment applications using natural and costeffective materials. This is the first-time white clay, Arabic gum, and marble powder were used in ceramic membranes. Two ceramic membranes were fabricated using an extrusion process: substrate A and substrate B. The JMP software (Version 15) was used to obtain the optimal recipes for the two substrates, which were white clay (62.7 %), silica flour (32.3 %), and Arabic gum (5 %) for substrate A and white clay (63 %), silica flour (26.8 %), and marble powder (10.2 %) for substrate B. Additionally, the effect of waste glass in the coating layer on the separation rate was examined. The ceramic membranes were analysed using various techniques, including X-ray fluorescence (XRF), X-ray diffraction (XRD), Fourier-transform infrared spectroscopy (FT-IR), laser diffraction particle size analysis, thermogravimetric analysis (TGA), and a universal testing machine. The morphologies of the membranes were observed using scan electron microscopy (SEM), and their chemical resistances were evaluated. The flux across the substrates was measured using a crossflow filtration system, and it was found that substrate B had a higher flux (116 L/m2 h) than substrate A (77 L/m2 h). This was probably due to its higher porosity (34 %) compared to substrate A (29 %). Substrate A, with a coating layer (CO-2), exhibited the highest removal efficiency of approximately 99.2 % for synthetic feed water composed of tap water and bentonite clay, with an average particle size of 1.1 μm and turbidity of 13 ± 0.2 NTU. The costs of ceramic membranes A and B were estimated to be approximately 51 and 47 USD/m2 , respectively. Their cost-effectiveness results from the use of low-cost materials that do not require high sintering temperatures. This study demonstrates that these ceramic membranes are not only affordable but also possess desirable properties for water treatment applications.

Type: Article
Title: Fabrication and characterization of coated ceramic membranes from natural sources for water treatment applications
Open access status: An open access version is available from UCL Discovery
DOI: 10.1016/j.memsci.2023.122226
Publisher version: https://doi.org/10.1016/j.memsci.2023.122226
Language: English
Additional information: © 2023 The Authors. Published by Elsevier B.V. This is an open access article under the CC BY license (http://creativecommons.org/licenses/by/4.0/).
Keywords: Ceramic membrane, White clay, Silica flour, Marble powder, Water treatment applications
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science > Dept of Chemical Engineering
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science > Dept of Civil, Environ and Geomatic Eng
URI: https://discovery.ucl.ac.uk/id/eprint/10180859
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