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Recent Advances in Ultralow-Pt-Loading Electrocatalysts for the Efficient Hydrogen Evolution

Guo, Fei; Macdonald, Thomas J; Sobrido, Ana Jorge; Liu, Longxiang; Feng, Jianrui; He, Guanjie; (2023) Recent Advances in Ultralow-Pt-Loading Electrocatalysts for the Efficient Hydrogen Evolution. Advanced Science , Article e2301098. 10.1002/advs.202301098. (In press). Green open access

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Abstract

Hydrogen production from water electrolysis provides a green and sustainable route. Platinum (Pt)-based materials have been regarded as efficient electrocatalysts for the hydrogen evolution reaction (HER). However, the large-scale commercialization of Pt-based catalysts suffers from the high cost. Therefore, ultralow-Pt-loading electrocatalysts, which can reach the balance of low cost and high HER performance, have attracted much attention. In this review, representative promising synthetic strategies, including wet chemistry, annealing, electrochemistry, photochemistry, and atomic layer deposition are summarized. Further, the interaction between different electrocatalyst components (transition metals and their derivatives) and Pt is discussed. Notably, this interaction can effectively accelerate the kinetics of the HER, enhancing the catalytic activity. At last, current challenges and future perspectives are briefly discussed.

Type: Article
Title: Recent Advances in Ultralow-Pt-Loading Electrocatalysts for the Efficient Hydrogen Evolution
Location: Germany
Open access status: An open access version is available from UCL Discovery
DOI: 10.1002/advs.202301098
Publisher version: https://doi.org/10.1002/advs.202301098
Language: English
Additional information: © 2023 The Authors. Advanced Science published by Wiley-VCH GmbH This is an open access article under the terms of the Creative Commons Attribution License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited.
Keywords: electrocatalysts, hydrogen evolution reaction, ultralow-Pt-loading
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science > Dept of Chemical Engineering
URI: https://discovery.ucl.ac.uk/id/eprint/10170189
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