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Improving Quantum Well Tube Homogeneity Using Strained Nanowire Heterostructures

Patel, N; Fonseka, HA; Zhang, Y; Church, S; Al-Abri, R; Sanchez, A; Liu, H; (2023) Improving Quantum Well Tube Homogeneity Using Strained Nanowire Heterostructures. ACS Applied Materials and Interfaces , 15 (8) pp. 10958-10964. 10.1021/acsami.2c22591. Green open access

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Abstract

Bottom-up grown nanostructures often suffer from significant dimensional inhomogeneity, and for quantum confined heterostructures, this can lead to a corresponding large variation in electronic properties. A high-throughput characterization methodology is applied to >15,000 nanoskived sections of highly strained GaAsP/GaAs radial core/shell quantum well heterostructures revealing high emission uniformity. While scanning electron microscopy shows a wide nanowire diameter spread of 540-60+60 nm, photoluminescence reveals a tightly bounded band-to-band transition energy of 1546-3+4 meV. A highly strained core/shell nanowire design is shown to reduce the dependence of emission on the quantum well width variation significantly more than in the unstrained case.

Type: Article
Title: Improving Quantum Well Tube Homogeneity Using Strained Nanowire Heterostructures
Location: United States
Open access status: An open access version is available from UCL Discovery
DOI: 10.1021/acsami.2c22591
Publisher version: https://doi.org/10.1021/acsami.2c22591
Language: English
Additional information: Copyright © 2023 The Authors. Published by American Chemical Society. This is an open access article under the CC BY 4.0 license Attribution 4.0 International (https://creativecommons.org/licenses/by/4.0/)
Keywords: heterostructure, high-throughput study, homogeneity, nanowire, quantum well, semiconductor
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science > Dept of Electronic and Electrical Eng
URI: https://discovery.ucl.ac.uk/id/eprint/10165776
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