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Effect of polydispersity and bubble clustering on the steady shear viscosity of dilute bubble suspensions in Newtonian media

Mitrou, S; Migliozzi, S; Angeli, P; Mazzei, L; (2023) Effect of polydispersity and bubble clustering on the steady shear viscosity of dilute bubble suspensions in Newtonian media. Presented at: 11th International Conference on Multiphase Flow, Kobe, Japan. Green open access

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Abstract

This work examines the steady shear viscosity of dilute polydisperse bubble suspensions generated in a mixture of mineral oil and span 80. We proved theoretically that, in polydisperse bubble suspensions, the shear-thinning behavior spans a capillary number (Ca) range between 0.01 and 100, instead of occurring at Ca~1, which is the case for monodisperse suspensions. However, for the effect of polydispersity to become apparent, the bubble size distribution should be bimodal, with very small and very large bubbles having similar volume fractions. In any other case, we can consider the polydisperse suspension as monodisperse, with a volume-weighted average diameter (d43). To confirm the theoretical results, we carried out steady shear rheological tests. Our measurements revealed an unexpected double power-law decay of the relative viscosity. To investigate this behavior further, we visualized the produced bubble suspensions under shear. The visualization experiments revealed that bubbles started forming clusters and threads at average capillary number around 0.01, where we observed the first decay of viscosity. CFD simulations confirmed that under the presence of bubble clusters and threads the fluid streamlines distort less, thus resulting in a decrease of the suspension viscosity. Consequently, we can attribute the first decay of the relative viscosity to the formation of bubble clusters and threads, proving that the novel shear-thinning behavior we observed is due to a combination of bubble clustering and deformation.

Type: Conference item (Presentation)
Title: Effect of polydispersity and bubble clustering on the steady shear viscosity of dilute bubble suspensions in Newtonian media
Event: 11th International Conference on Multiphase Flow
Location: Kobe, Japan
Dates: 02 - 07 April 2023
Open access status: An open access version is available from UCL Discovery
Publisher version: http://www.jsmf.gr.jp/icmf2022/
Language: English
Keywords: Bubble suspension, Steady shear viscosity, Bubble clustering
UCL classification: UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science > Dept of Chemical Engineering
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL
URI: https://discovery.ucl.ac.uk/id/eprint/10157880
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