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An Ultra-Thin Near-Perfect Absorber via Block Copolymer Engineered Metasurfaces

Cummins, C; Flamant, Q; Dwivedi, R; Alvarez-Fernandez, A; Demazy, N; Bentaleb, A; Pound-Lana, G; ... Ponsinet, V; + view all (2022) An Ultra-Thin Near-Perfect Absorber via Block Copolymer Engineered Metasurfaces. Journal of Colloid and Interface Science , 609 pp. 375-383. 10.1016/j.jcis.2021.11.163. Green open access

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Abstract

Producing ultrathin light absorber layers is attractive towards the integration of lightweight planar components in electronic, photonic, and sensor devices. In this work, we report the experimental demonstration of a thin gold (Au) metallic metasurface with near-perfect visible absorption (∼95 %). Au nanoresonators possessing heights from 5 − 15 nm with sub-50 nm diameters were engineered by block copolymer (BCP) templating. The Au nanoresonators were fabricated on an alumina (Al2O3) spacer layer and a reflecting Au mirror, in a film-coupled nanoparticle design. The BCP nanopatterning strategy to produce desired heights of Au nanoresonators was tailored to achieve near-perfect absorption at ≈ 600 nm. The experimental insight described in this work is a step forward towards realizing large area flat optics applications derived from subwavelength-thin metasurfaces.

Type: Article
Title: An Ultra-Thin Near-Perfect Absorber via Block Copolymer Engineered Metasurfaces
Location: United States
Open access status: An open access version is available from UCL Discovery
DOI: 10.1016/j.jcis.2021.11.163
Publisher version: https://doi.org/10.1016/j.jcis.2021.11.163
Language: English
Additional information: This version is the author accepted manuscript. For information on re-use, please refer to the publisher’s terms and conditions.
Keywords: Science & Technology, Physical Sciences, Chemistry, Physical, Chemistry, Block copolymers, Metasurfaces, Perfect absorbers, Nanoresonators, Flat optics, ARRAYS
UCL classification: UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science > Dept of Chemical Engineering
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL
URI: https://discovery.ucl.ac.uk/id/eprint/10151018
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