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Robustness of Basal-Plane Antiferromagnetic Order and the J(eff)=1/2 State in Single-Layer Iridate Spin-Orbit Mott Insulators

Boseggia, S; Springell, R; Walker, HC; Ronnow, HM; Rueegg, C; Okabe, H; Isobe, M; ... McMorrow, DF; + view all (2013) Robustness of Basal-Plane Antiferromagnetic Order and the J(eff)=1/2 State in Single-Layer Iridate Spin-Orbit Mott Insulators. Physical Review Letters , 110 (11) , Article 117207. 10.1103/PhysRevLett.110.117207. Green open access

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Abstract

The magnetic structure and electronic ground state of the layered perovskite Ba 2 IrO 4 have been investigated using x-ray resonant magnetic scattering. Our results are compared with those for Sr 2 IrO 4 , for which we provide supplementary data on its magnetic structure. We find that the dominant, long-range antiferromagnetic order is remarkably similar in the two compounds and that the electronic ground state in Ba 2 IrO 4 , deduced from an investigation of the x-ray resonant magnetic scattering L 3 / L 2 intensity ratio, is consistent with a J eff = 1 / 2 description. The robustness of these two key electronic properties to the considerable structural differences between the Ba and Sr analogues is discussed in terms of the enhanced role of the spin-orbit interaction in 5 d transition metal oxides.

Type: Article
Title: Robustness of Basal-Plane Antiferromagnetic Order and the J(eff)=1/2 State in Single-Layer Iridate Spin-Orbit Mott Insulators
Open access status: An open access version is available from UCL Discovery
DOI: 10.1103/PhysRevLett.110.117207
Publisher version: https://doi.org/10.1103/PhysRevLett.110.117207
Language: English
Additional information: This version is the author accepted manuscript. For information on re-use, please refer to the publisher’s terms and conditions.
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences > London Centre for Nanotechnology
URI: https://discovery.ucl.ac.uk/id/eprint/10134049
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