Rawlings, JMC; Wilson, TG; Williams, DA; (2019) A gas-phase primordial origin of O-2 in comet 67P/Churyumov-Gerasimenko. Monthly Notices of the Royal Astronomical Society , 486 (1) pp. 10-20. 10.1093/mnras/stz689.

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Abstract

Recent observations made by the Rosetta/ROSINA instrument have detected molecular oxygen in the coma of comet 67P/Churyumov-Gerasimenko with abundances at the 1–10 per cent level relative to H2O. Previous studies have indicated that the likely origin of the O2 may be surface chemistry of primordial (dark cloud) origin, requiring somewhat warmer, denser, and extreme H-atom poor conditions than are usually assumed. In this study, we propose a primordial gas-phase origin for the O2 that is subsequently frozen and effectively hidden until the ice mantles are sublimated in the comet’s coma. Our study presents results from a three-phase astrochemical model that simulates the chemical evolution of ices in the primordial dark cloud phase, its gravitational collapse, and evolution in the early protosolar nebula. We find that the O2 abundance can be produced and is fairly robust to the choice of the free parameters. Good matches for the O2:H2O ratio and, to a lesser extent, the N2:CO and CO:H2O ratios are obtained, but the models significantly overproduce N2. We speculate that the low value of N2:O2 that is observed is a consequence of the specific thermal history of the comet.

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