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Correlation between Cu ion migration behaviour and deNO x activity in Cu-SSZ-13 for the standard NH 3 -SCR reaction

Beale, AM; Lezcano-Gonzalez, I; Slawinksi, WA; Wragg, DS; (2016) Correlation between Cu ion migration behaviour and deNO x activity in Cu-SSZ-13 for the standard NH 3 -SCR reaction. Chemical Communications , 52 (36) pp. 6170-6173. 10.1039/C6CC00513F. Green open access

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Abstract

Here we present the results of a synchrotron-based in situ, time-resolved PXRD study during activation of two Cu-SSZ-13 catalysts under O2/He and one during standard NH3-SCR reaction conditions to obtain insight into the behaviour of Cu ions. The results obtained indicate that deNOx activity is inexorably linked with occupancy of the zeolite 6r.

Type: Article
Title: Correlation between Cu ion migration behaviour and deNO x activity in Cu-SSZ-13 for the standard NH 3 -SCR reaction
Open access status: An open access version is available from UCL Discovery
DOI: 10.1039/C6CC00513F
Publisher version: http://dx.doi.org/10.1039/C6CC00513F
Additional information: © The Royal Society of Chemistry 2016. This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences > Dept of Chemistry
URI: https://discovery.ucl.ac.uk/id/eprint/1507874
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