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Magnetic structure and field-dependent magnetic phase diagram of Ni2In-type PrCuSi

Nair, HS; Kumar, CMN; Adroja, DT; Ritter, C; Wills, AS; Kockelmann, WA; Deen, PP; ... Strydom, AM; + view all (2018) Magnetic structure and field-dependent magnetic phase diagram of Ni2In-type PrCuSi. Journal of Physics: Condensed Matter , 30 (43) , Article 435803. 10.1088/1361-648X/aae28d. Green open access

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Abstract

The magnetic structure of the ternary equiatomic intermetallic compound PrCuSi is investigated using neutron powder diffraction experiments in 0 T as well as in external magnetic fields up to 2 T. The PrCuSi compound crystallizes in the hexagonal Ni2In-type structure, in the space group P63/mmc. In this structure, cationic ordering of Cu and Si takes place. The antiferromagnetic phase transition in the Pr sublattice takes place at K in 0 T. Under an external magnetic field of 2 T, a field-induced ferromagnetic phase is observed. Magnetoelastic coupling is evidenced by an increase in the unit cell volume. Clear signatures of a mixed antiferromagnetic and ferromagnetic phase in weak, intermediate fields, 0.4–0.8 T, are obtained from the present study. Using the present set of experimental data, we construct the H  −  T phase diagram of PrCuSi.

Type: Article
Title: Magnetic structure and field-dependent magnetic phase diagram of Ni2In-type PrCuSi
Open access status: An open access version is available from UCL Discovery
DOI: 10.1088/1361-648X/aae28d
Publisher version: http://dx.doi.org/10.1088/1361-648X/aae28d
Language: English
Additional information: This version is the author accepted manuscript. For information on re-use, please refer to the publisher’s terms and conditions.
Keywords: Science & Technology, Physical Sciences, Physics, Condensed Matter, Physics, antiferromagnet, PrCuSi, magnetostructural effect, field induced ferromagnetism, NEUTRON-DIFFRACTION, GERMANIDES, TRANSITION, SILICIDES, TB
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences > Dept of Chemistry
URI: https://discovery.ucl.ac.uk/id/eprint/10059825
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