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Light-driven generation of chlorine and hydrogen from brine using highly selective Ru/Ti oxide redox catalysts

McCafferty, L; O'Rourke, C; Mills, A; Kafizas, A; Parkin, IP; Darr, JA; (2017) Light-driven generation of chlorine and hydrogen from brine using highly selective Ru/Ti oxide redox catalysts. Sustainable Energy Fuels , 1 (2) pp. 254-257. 10.1039/C6SE00057F. Green open access

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Abstract

Ultrafine ruthenium–titanium oxide catalysts were directly produced using a continuous hydrothermal flow synthesis process and assessed as chloride oxidation catalysts. Selectivity towards chlorine (over oxygen) evolution was shown to generally increase with decreasing ruthenium content. The optimum catalyst was then used to make an anode for a light-driven brine-splitting demonstrator device to produce hydrogen and chlorine gases.

Type: Article
Title: Light-driven generation of chlorine and hydrogen from brine using highly selective Ru/Ti oxide redox catalysts
Open access status: An open access version is available from UCL Discovery
DOI: 10.1039/C6SE00057F
Publisher version: http://doi.org/10.1039/C6SE00057F
Language: English
Additional information: This journal is © The Royal Society of Chemistry 2017. This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
UCL classification: UCL > Provost and Vice Provost Offices
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences > Dept of Chemistry
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences > MAPS Faculty Office
UCL > Provost and Vice Provost Offices > VP Innovation and Enterprise
UCL > Provost and Vice Provost Offices > VP Innovation and Enterprise > Business and Innovation Partnerships
URI: https://discovery.ucl.ac.uk/id/eprint/1543142
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