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Structure of Self-Assembled Mn Atom Chains on Si(001)

Villarreal, R; Longobardi, M; Köster, SA; Kirkham, CJ; Bowler, D; Renner, C; (2015) Structure of Self-Assembled Mn Atom Chains on Si(001). Physical Review Letters , 115 (25) , Article 256104. 10.1103/PhysRevLett.115.256104. Green open access

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Abstract

Mn has been found to self-assemble into atomic chains running perpendicular to the surface dimer reconstruction on Si(001). They differ from other atomic chains by a striking asymmetric appearance in filled state scanning tunneling microscopy (STM) images. This has prompted complicated structural models involving up to three Mn atoms per chain unit. Combining STM, atomic force microscopy, and density functional theory we find that a simple necklacelike chain of single Mn atoms reproduces all their prominent features, including their asymmetry not captured by current models. The upshot is a remarkably simpler structure for modeling the electronic and magnetic properties of Mn atom chains on Si(001).

Type: Article
Title: Structure of Self-Assembled Mn Atom Chains on Si(001)
Open access status: An open access version is available from UCL Discovery
DOI: 10.1103/PhysRevLett.115.256104
Publisher version: http://dx.doi.org/10.1103/PhysRevLett.115.256104
Language: English
Additional information: Copyright © 2015 American Physical Society.
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences > Dept of Physics and Astronomy
URI: https://discovery.ucl.ac.uk/id/eprint/1503986
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