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Pressure-tuned spin and charge ordering in an itinerant antiferromagnet

Feng, Y; Jaramillo, R; Srajer, G; Lang, JC; Islam, Z; Somayazulu, MS; Shpyrko, OG; ... Rosenbaum, TF; + view all (2007) Pressure-tuned spin and charge ordering in an itinerant antiferromagnet. PHYS REV LETT , 99 (13) , Article 137201. 10.1103/PhysRevLett.99.137201. Green open access

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Abstract

Elemental chromium orders antiferromagnetically near room temperature, but the ordering temperature can be driven to zero by applying large pressures. We combine diamond anvil cell and synchrotron x-ray diffraction techniques to measure directly the spin and charge order in the pure metal at the approach to its quantum critical point. Both spin and charge order are suppressed exponentially with pressure, well beyond the region where disorder cuts off such a simple evolution, and they maintain a harmonic scaling relationship over decades in scattering intensity. By comparing the development of the order parameter with that of the magnetic wave vector, it is possible to ascribe the destruction of antiferromagnetism to the growth in electron kinetic energy relative to the underlying magnetic exchange interaction.

Type: Article
Title: Pressure-tuned spin and charge ordering in an itinerant antiferromagnet
Open access status: An open access version is available from UCL Discovery
DOI: 10.1103/PhysRevLett.99.137201
Publisher version: http://dx.doi.org/10.1103/PhysRevLett.99.137201
Language: English
Additional information: © 2007 The American Physical Society
Keywords: QUANTUM CRITICAL-POINT, MAGNETIC EXCITATIONS, NEEL TRANSITION, DENSITY WAVES, CHROMIUM, ALLOYS, SCATTERING, HEAVY, TEMPERATURE, DEPENDENCE
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences
URI: https://discovery.ucl.ac.uk/id/eprint/129324
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