Ye, Jingyun;
Dimitratos, Nikolaos;
Rossi, Liane M;
Thonemann, Nils;
Beale, Andrew M;
Wojcieszak, Robert;
(2025)
Hydrogenation of CO₂ for sustainable fuel and chemical production.
Science
, 387
(6737)
, Article eadn9388. 10.1126/science.adn9388.
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Abstract
Catalytic carbon dioxide (CO2) hydrogenation is a potential route for producing sustainable fuels and chemicals, but existing catalysts need improvement. In particular, identifying active sites and understanding the interaction between components and the dynamic behavior of the participant species remain unclear. This fundamental knowledge is essential for the design of more efficient and stable catalysts. Because the nature of the active site (metal, oxide, carbide) is the main factor that determines the catalytic activity of the catalysts, this Review focuses on various types of heterogeneous catalysts that have been recently reported in the literature as efficient for CO2 conversion to C1 [carbon monoxide (CO), methanol (CH3OH), methane (CH4)], and higher hydrocarbons. We focus on establishing key connections between active-site structures and selectivity, regardless of catalyst composition.
| Type: | Article |
|---|---|
| Title: | Hydrogenation of CO₂ for sustainable fuel and chemical production |
| Location: | United States |
| Open access status: | An open access version is available from UCL Discovery |
| DOI: | 10.1126/science.adn9388 |
| Publisher version: | https://doi.org/10.1126/science.adn9388 |
| Language: | English |
| Additional information: | This version is the author accepted manuscript. For information on re-use, please refer to the publisher’s terms and conditions. |
| UCL classification: | UCL UCL > Provost and Vice Provost Offices > UCL BEAMS UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences > Dept of Chemistry |
| URI: | https://discovery.ucl.ac.uk/id/eprint/10208068 |
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