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Hopping protons in supramolecular catalysis

Haynes, Cally JE; von Krbek, Larissa KS; (2022) Hopping protons in supramolecular catalysis. Nature Chemistry , 14 (9) pp. 969-971. 10.1038/s41557-022-01024-w. Green open access

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Abstract

Supramolecular catalysis can emulate many features of enzymatic transformations. Now, a complex proton wire mechanism — enabling the dual activation of a nucleophile and an electrophile through reciprocal proton transfer — has been shown to operate during the β-glycosylation of sugars within a self-assembled capsule.

Type: Article
Title: Hopping protons in supramolecular catalysis
Location: England
Open access status: An open access version is available from UCL Discovery
DOI: 10.1038/s41557-022-01024-w
Publisher version: https://doi.org/10.1038/s41557-022-01024-w
Language: English
Additional information: This version is the author accepted manuscript. For information on re-use, please refer to the publisher’s terms and conditions.
Keywords: Catalysis, Models, Molecular, Protons
UCL classification: UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences > Dept of Chemistry
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL
URI: https://discovery.ucl.ac.uk/id/eprint/10156904
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