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Biodegradable Polyurethane Fiber-Based Strain Sensor with a Broad Sensing Range and High Sensitivity for Human Motion Monitoring

Liu, Zhanxu; Li, Chenchen; Zhang, Xiaofeng; Zhou, Bangze; Wen, Shipeng; Zhou, Yanfen; Chen, Shaojuan; ... Zhou, Fenglei; + view all (2022) Biodegradable Polyurethane Fiber-Based Strain Sensor with a Broad Sensing Range and High Sensitivity for Human Motion Monitoring. ACS Sustainable Chemistry and Engineering , 10 (27) pp. 8788-8798. 10.1021/acssuschemeng.2c01171. Green open access

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Abstract

To date, a majority of polymer-based wearable flexible strain sensors are non-biodegradable, which inevitably causes environmental pollution at the end of their service life. In this work, biodegradable polyurethane (BPU) was synthesized and then processed with carbon nanotubes (CNTs) via wet spinning into BPU/CNT composite fibers used as strain sensors. The synthesized BPU showed excellent biodegradability with a 19.45% weight loss in 42 days in a phosphate buffered saline (PBS) solution. Compared with previously reported strain sensors made from silk, cellulose, and polylactic acid, the BPU/12%CNT fibers achieved a much wider strain-sensing range (0–250%) and a high sensitivity (gauge factors of 15 at 100% strain and of 2468 at 250% strain respectively) while exhibiting reliable stability. These properties allow strain sensors based on BPU/CNT fibers and knitted fabric to be successfully used for monitoring various human motions. Moreover, biodegradability of the BPU/CNT strain sensor in a PBS solution was verified. In consequence, this work provides insights into the development of biodegradable wearable electronic devices.

Type: Article
Title: Biodegradable Polyurethane Fiber-Based Strain Sensor with a Broad Sensing Range and High Sensitivity for Human Motion Monitoring
Open access status: An open access version is available from UCL Discovery
DOI: 10.1021/acssuschemeng.2c01171
Publisher version: https://doi.org/10.1021/acssuschemeng.2c01171
Language: English
Additional information: This version is the author accepted manuscript. For information on re-use, please refer to the publisher’s terms and conditions.
Keywords: Biodegradability, polyurethane, fiber, strain sensor, carbon nanotubes
UCL classification: UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science > Dept of Med Phys and Biomedical Eng
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL
URI: https://discovery.ucl.ac.uk/id/eprint/10153429
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