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Identification and manipulation of dynamic active site deficiency-induced competing reactions in electrocatalytic oxidation processes

Lin, Runjia; Kang, Liqun; Zhao, Tianqi; Feng, Jianrui; Celorrio, Veronica; Zhang, Guohui; Cibin, Giannantonio; ... He, Guanjie; + view all (2022) Identification and manipulation of dynamic active site deficiency-induced competing reactions in electrocatalytic oxidation processes. Energy & Environmental Science 10.1039/d1ee03522c. (In press). Green open access

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Abstract

A detrimental competition between the urea oxidation reaction (UOR) and oxygen evolution reaction is identified. Strategies are proposed to alleviate such competition and boost the performance of the UOR and other organic compound oxidation reactions.

Type: Article
Title: Identification and manipulation of dynamic active site deficiency-induced competing reactions in electrocatalytic oxidation processes
Open access status: An open access version is available from UCL Discovery
DOI: 10.1039/d1ee03522c
Publisher version: https://doi.org/10.1039/D1EE03522C
Language: English
Additional information: This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Keywords: Science & Technology, Physical Sciences, Technology, Life Sciences & Biomedicine, Chemistry, Multidisciplinary, Energy & Fuels, Engineering, Chemical, Environmental Sciences, Chemistry, Engineering, Environmental Sciences & Ecology, OXYGEN EVOLUTION, CATALYSTS, EFFICIENT, RECONSTRUCTION, HYDROGEN, PERFORMANCE, REDUCTION, OXIDES
UCL classification: UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science > Dept of Chemical Engineering
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences > Dept of Chemistry
URI: https://discovery.ucl.ac.uk/id/eprint/10147090
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