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Design of Scalable, Next-Generation Thick Electrodes: Opportunities and Challenges

Boyce, AM; Cumming, DJ; Huang, C; Zankowski, SP; Grant, PS; Brett, DJL; Shearing, PR; (2021) Design of Scalable, Next-Generation Thick Electrodes: Opportunities and Challenges. ACS Nano , 15 (12) pp. 18624-18632. 10.1021/acsnano.1c09687. Green open access

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Abstract

Lithium-ion battery electrodes are on course to benefit from current research in structure re-engineering to allow for the implementation of thicker electrodes. Increasing the thickness of a battery electrode enables significant improvements in gravimetric energy density while simultaneously reducing manufacturing costs. Both metrics are critical if the transition to sustainable transport systems is to be fully realized commercially. However, significant barriers exist that prevent the use of such microstructures: performance issues, manufacturing challenges, and scalability all remain open areas of research. In this Perspective, we discuss the challenges in adapting current manufacturing processes for thick electrodes and the opportunities that pore engineering presents in order to design thicker and better electrodes while simultaneously considering long-term performance and scalability.

Type: Article
Title: Design of Scalable, Next-Generation Thick Electrodes: Opportunities and Challenges
Location: United States
Open access status: An open access version is available from UCL Discovery
DOI: 10.1021/acsnano.1c09687
Publisher version: https://doi.org/10.1021/acsnano.1c09687
Language: English
Additional information: This version is the author accepted manuscript. For information on re-use, please refer to the publisher’s terms and conditions.
Keywords: Batteries, Electrodes, Manufacturing, Materials, Thickness
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science > Dept of Chemical Engineering
URI: https://discovery.ucl.ac.uk/id/eprint/10140176
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