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Novel sinuous band microelectrode array for electrochemical amperometric sensing

Li, Y; Yin, S; Jiang, N; Li, X; Liu, C; Li, J; Liu, Y; (2021) Novel sinuous band microelectrode array for electrochemical amperometric sensing. Electrochemistry Communications , 133 , Article 107159. 10.1016/j.elecom.2021.107159. Green open access

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Abstract

Pursuing a higher response signal is the core challenge in improving the detection performance of a microelectrode-based amperometric electrochemical sensor. Band microelectrode arrays (bMEAs) are attractive due to their high response current and economical fabrication process. However, further amplifying the response current by arranging the array more compactly or increasing its size is generally hindered by the shielding effect or the restricted construction region. A novel array of sinuous band microelectrodes (sbMEA) is proposed, produced by deforming a bMEA by tilting and bending. Its response and diffusion characteristics are simulated and analyzed. The effects of structural parameters on its performance are revealed, and their optimal value is deduced. The simulation demonstrates that a sbMEA can generate a larger current than a MEA of traditional shape. Production of such a sbMEA does not involve any additional fabrication costs compared with a bMEA. Cyclic voltammetry (CV) tests with potassium ferrocyanide solution verify the theoretical performance of the sbMEA, and a 10% higher current was obtained compared to the corresponding bMEA.

Type: Article
Title: Novel sinuous band microelectrode array for electrochemical amperometric sensing
Open access status: An open access version is available from UCL Discovery
DOI: 10.1016/j.elecom.2021.107159
Publisher version: https://doi.org/10.1016/j.elecom.2021.107159
Language: English
Additional information: © 2021 Published by Elsevier Ltd. This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/)
Keywords: Amperometric, Tilt, Bend, Sinuous band microelectrode
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science > Dept of Mechanical Engineering
URI: https://discovery.ucl.ac.uk/id/eprint/10138705
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