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Structural Sensitivity of the Water Gas Shift Reaction on Platinum Surfaces

Stamatakis, M; Chen, Y; Vlachos, DG; (2011) Structural Sensitivity of the Water Gas Shift Reaction on Platinum Surfaces. Presented at: North American Catalysis Society 22nd North American Meeting, Detroit, MI, USA. Green open access

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Abstract

We investigate the structure sensitivity of the water-gas shift reaction on Pt, showing that the stepped surfaces Pt(322) and Pt(211) exhibit much higher activities than Pt(111). Statistical analysis of reaction occurrence elucidates the contribution of steps and terraces on the observed rates, indentifying the active sites for each elementary reaction.

Type: Conference item (UNSPECIFIED)
Title: Structural Sensitivity of the Water Gas Shift Reaction on Platinum Surfaces
Event: North American Catalysis Society 22nd North American Meeting
Location: Detroit, MI, USA
Dates: 05 June 2011 - 10 June 2011
Open access status: An open access version is available from UCL Discovery
Publisher version: https://nam.confex.com/nam/2011/webprogram/Paper43...
Language: English
Additional information: This version is the author accepted manuscript. For information on re-use, please refer to the publisher’s terms and conditions.
UCL classification: UCL
UCL > Provost and Vice Provost Offices
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science > Dept of Chemical Engineering
URI: https://discovery.ucl.ac.uk/id/eprint/10133578
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