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Mercury atmospheric emission, deposition and isotopic fingerprinting from major coal-fired power plants in Australia: Insights from palaeo-environmental analysis from sediment cores

Schneider, L; Rose, NL; Myllyvirta, L; Haberle, S; Lintern, A; Yuan, J; Sinclair, D; ... Sun, R; + view all (2021) Mercury atmospheric emission, deposition and isotopic fingerprinting from major coal-fired power plants in Australia: Insights from palaeo-environmental analysis from sediment cores. Environmental Pollution , 287 (117596) 10.1016/j.envpol.2021.117596. Green open access

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Abstract

Despite Australia's high reliance on coal for electricity generation, no study has addressed the extent to which mercury (Hg) deposition has increased since the commissioning of coal-fired power plants. We present stratigraphic data from lake sediments in the Hunter Valley (New South Wales) and Latrobe Valley (Victoria), where a significant proportion of Australia's electricity is generated via coal combustion. Mercury deposition in lake sediments increased in the 1970s with the commissioning of coal-fired power plants, by a factor of 2.9-times in sediments of Lake Glenbawn (Hunter Valley) and 14-times in Traralgon Reservoir (Latrobe Valley). Sediments deposited after the commissioning of power plants have distinct Hg isotope compositions, similar to those of combusted coals. Mercury emission, estimated using an atmospheric model (CALPUFF), was higher in the Latrobe Valley than in the Hunter Valley. This is a result of higher Hg concentrations in lignite coal, lax regulation and older pollution-control technologies adopted by coal-fired power plants in the Latrobe Valley. Near-source deposition of Hg in Australia is significantly higher than North America and Europe, where better emission controls (e.g. wet flue gas desulfurization) have been in effect for decades. The challenge for Australia in years to come will be to ratify the Minamata Convention and develop better regulation policies to reduce Hg emissions.

Type: Article
Title: Mercury atmospheric emission, deposition and isotopic fingerprinting from major coal-fired power plants in Australia: Insights from palaeo-environmental analysis from sediment cores
Open access status: An open access version is available from UCL Discovery
DOI: 10.1016/j.envpol.2021.117596
Publisher version: https://doi.org/10.1016/j.envpol.2021.117596
Language: English
Additional information: This version is the author accepted manuscript. For information on re-use, please refer to the publisher’s terms and conditions.
Keywords: CALPUFF, Mercury isotope, Bag filter, Electrostatic precipitator, Minamata convention
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL SLASH
UCL > Provost and Vice Provost Offices > UCL SLASH > Faculty of S&HS
UCL > Provost and Vice Provost Offices > UCL SLASH > Faculty of S&HS > Dept of Geography
URI: https://discovery.ucl.ac.uk/id/eprint/10130345
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