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Mechanochemical reactivity inhibited, prohibited and reversed by liquid additives: examples from crystal-form screens

Arhangelskis, M; Bučar, D-K; Bordignon, S; Chierotti, MR; Stratford, SA; Voinovich, D; Jones, W; (2021) Mechanochemical reactivity inhibited, prohibited and reversed by liquid additives: examples from crystal-form screens. Chemical Science 10.1039/d0sc05071g. (In press). Green open access

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Abstract

We demonstrate that liquid additives can exert inhibitive or prohibitive effects on the mechanochemical formation of multi-component molecular crystals, and report that certain additives unexpectedly prompt the dismantling of such solids into physical mixtures of their constituents. Computational methods were employed in an attempt to identify possible reasons for these previously unrecognised effects of liquid additives on mechanochemical transformations.

Type: Article
Title: Mechanochemical reactivity inhibited, prohibited and reversed by liquid additives: examples from crystal-form screens
Open access status: An open access version is available from UCL Discovery
DOI: 10.1039/d0sc05071g
Publisher version: https://doi.org/10.1039/D0SC05071G
Language: English
Additional information: Open Access Article. This Open Access Article is licensed under a Creative Commons Attribution-Non Commercial 3.0 Unported Licence
UCL classification: UCL
UCL > Provost and Vice Provost Offices
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences > Dept of Chemistry
URI: https://discovery.ucl.ac.uk/id/eprint/10120165
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