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Carbon nanotube-reduced graphene oxide fiber with high torsional strength from rheological hierarchy control

Eom, W; Lee, E; Lee, SH; Sung, TH; Clancy, AJ; Lee, WJ; Han, TH; (2021) Carbon nanotube-reduced graphene oxide fiber with high torsional strength from rheological hierarchy control. Nature Communications , 12 (1) , Article 396. 10.1038/s41467-020-20518-0. (In press). Green open access

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Abstract

High torsional strength fibers are of practical interest for applications such as artificial muscles, electric generators, and actuators. Herein, we maximize torsional strength by understanding, measuring, and overcoming rheological thresholds of nanocarbon (nanotube/graphene oxide) dopes. The formed fibers show enhanced structure across multiple length scales, modified hierarchy, and improved mechanical properties. In particular, the torsional properties were examined, with high shear strength (914 MPa) attributed to nanotubes but magnified by their structure, intercalating graphene sheets. This design approach has the potential to realize the hierarchical dimensional hybrids, and may also be useful to build the effective network structure of heterogeneous materials.

Type: Article
Title: Carbon nanotube-reduced graphene oxide fiber with high torsional strength from rheological hierarchy control
Location: England
Open access status: An open access version is available from UCL Discovery
DOI: 10.1038/s41467-020-20518-0
Publisher version: http://dx.doi.org/10.1038/s41467-020-20518-0
Language: English
Additional information: Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/ licenses/by/4.0/. © The Author(s) 2021
Keywords: Condensed-matter physics, Nanoscale materials, Soft materials
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences > Dept of Chemistry
URI: https://discovery.ucl.ac.uk/id/eprint/10119390
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