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Unusual breathing behavior of optically excited barium titanate nanocrystals

Diao, J; Cherukara, M; Harder, R; Huang, X; Zhang, F; Chen, B; Ulvestad, A; ... Robinson, I; + view all (2020) Unusual breathing behavior of optically excited barium titanate nanocrystals. Crystals , 10 (5) , Article 365. 10.3390/cryst10050365. Green open access

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Abstract

Coherent X-ray diffraction patterns were recorded by using an X-ray free-electron laser to illuminate barium titanate nanocrystals as a function of time delay after laser excitation. Rather than seeing any significant thermal expansion effects, the diffraction peaks were found to move perpendicular to the momentum transfer direction. This suggests a laser driven rotation of the crystal lattice, which is delayed by the aggregated state of the crystals. Internal deformations associated with crystal contacts were also observed.

Type: Article
Title: Unusual breathing behavior of optically excited barium titanate nanocrystals
Open access status: An open access version is available from UCL Discovery
DOI: 10.3390/cryst10050365
Publisher version: https://doi.org/10.3390/cryst10050365
Language: English
Additional information: This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/
Keywords: X-ray pump-probe; coherent imaging; ferroelectric oxide
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences > Dept of Physics and Astronomy
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences > London Centre for Nanotechnology
URI: https://discovery.ucl.ac.uk/id/eprint/10098219
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