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Canted antiferromagnetic order in the kagome material Sr-vesignieite

Verrier, A; Bert, F; Parent, J-M; El-Amine, M; Orain, JC; Boldrin, D; Wills, AS; ... Quilliam, JA; + view all (2020) Canted antiferromagnetic order in the kagome material Sr-vesignieite. Physical Review B , 101 (5) , Article 054425. 10.1103/PhysRevB.101.054425. Green open access

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Abstract

We report 51 V NMR, muon spin rotation, and zero-applied-field 63 , 65 Cu NMR measurements on powder samples of Sr-vesignieite, SrCu 3 V 2 O 8 ( OH ) 2 , a S = 1 / 2 nearly kagome Heisenberg antiferromagnet. Our results demonstrate that the ground state is a q = 0 magnetic structure with spins canting either in or out of the kagome plane, giving rise to weak ferromagnetism. We determine the size of ordered moments and the angle of canting for different possible q = 0 structures and orbital scenarios, thereby providing insight into the role of the Dzyaloshinskii-Moriya interaction in this material.

Type: Article
Title: Canted antiferromagnetic order in the kagome material Sr-vesignieite
Open access status: An open access version is available from UCL Discovery
DOI: 10.1103/PhysRevB.101.054425
Publisher version: https://doi.org/10.1103/PhysRevB.101.054425
Language: English
Additional information: This version is the version of record. For information on re-use, please refer to the publisher’s terms and conditions.
Keywords: Science & Technology, Technology, Physical Sciences, Materials Science, Multidisciplinary, Physics, Applied, Physics, Condensed Matter, Materials Science, Physics, LIQUID GROUND-STATE, ORBITAL FRUSTRATION
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences > Dept of Chemistry
URI: https://discovery.ucl.ac.uk/id/eprint/10091825
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