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Pressure effects on the structural and superconducting transitions in La₃Co₄Sn₁₃

Mendonça-Ferreira, L; Carneiro, FB; Fontes, MB; Baggio-Saitovitch, E; Veiga, LS; Mardegan, JRL; Strempfer, J; ... Bittar, EM; + view all (2019) Pressure effects on the structural and superconducting transitions in La₃Co₄Sn₁₃. Journal of Alloys and Compounds , 773 pp. 34-39. 10.1016/j.jallcom.2018.09.236. Green open access

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Abstract

La3Co4Sn13 is a superconducting material with transition temperature at Tc = 2.70 K, which presents a superlattice structural transition at T ∗ ≃ 150 K, a common feature for this class of compounds. However, for this material, it is not clear that at T ∗ the lattice distortions arise from a charge density wave (CDW) or from a distinct microscopic origin. Interestingly, it has been suggested in isostructural non-magnetic intermetallic compounds that T ∗ can be suppressed to zero temperature, by combining chemical and external pressure, and a quantum critical point is argued to be observed near these critical doping/pressure. Our study shows that application of pressure on single-crystalline La3Co4Sn13 enhances Tc and decreases T ∗ . We observe thermal hysteresis loops for cooling/heating cycles around T ∗ for P & 0.6 GPa, in electrical resistivity measurements, which are not seen in x-ray diffraction data. The hysteresis in electrical measurements may be due to the pinning of the CDW phase to impurities/defects, while the superlattice structural transition maintains its ambient pressure second-order transition nature under pressure. From our experiments we estimate that T ∗ vanishes at around 5.5 GPa, though no quantum critical behavior is observed up to 2.53 GPa.

Type: Article
Title: Pressure effects on the structural and superconducting transitions in La₃Co₄Sn₁₃
Open access status: An open access version is available from UCL Discovery
DOI: 10.1016/j.jallcom.2018.09.236
Publisher version: https://doi.org/10.1016/j.jallcom.2018.09.236
Language: English
Additional information: This version is the author accepted manuscript. For information on re-use, please refer to the publisher’s terms and conditions.
Keywords: Pressure effects, La₃Co₄Sn₁₃, Superconductivity, Electrical resistivity, Synchrotron x-ray diffraction
UCL classification: UCL
UCL > Provost and Vice Provost Offices
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences > London Centre for Nanotechnology
URI: https://discovery.ucl.ac.uk/id/eprint/10085886
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