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Quenching of dynamic nuclear polarization by spin–orbit coupling in GaAs quantum dots

Nichol, JM; Harvey, SP; Shulman, MD; Pal, A; Umansky, V; Rashba, EI; Halperin, BI; (2015) Quenching of dynamic nuclear polarization by spin–orbit coupling in GaAs quantum dots. Nature Communications , 6 , Article 7682. 10.1038/ncomms8682. Green open access

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Abstract

The central-spin problem is a widely studied model of quantum decoherence. Dynamic nuclear polarization occurs in central-spin systems when electronic angular momentum is transferred to nuclear spins and is exploited in quantum information processing for coherent spin manipulation. However, the mechanisms limiting this process remain only partially understood. Here we show that spin–orbit coupling can quench dynamic nuclear polarization in a GaAs quantum dot, because spin conservation is violated in the electron–nuclear system, despite weak spin–orbit coupling in GaAs. Using Landau–Zener sweeps to measure static and dynamic properties of the electron spin–flip probability, we observe that the size of the spin–orbit and hyperfine interactions depends on the magnitude and direction of applied magnetic field. We find that dynamic nuclear polarization is quenched when the spin–orbit contribution exceeds the hyperfine, in agreement with a theoretical model. Our results shed light on the surprisingly strong effect of spin–orbit coupling in central-spin systems.

Type: Article
Title: Quenching of dynamic nuclear polarization by spin–orbit coupling in GaAs quantum dots
Open access status: An open access version is available from UCL Discovery
DOI: 10.1038/ncomms8682
Publisher version: https://doi.org/10.1038/ncomms8682
Language: English
Additional information: This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
Keywords: Quantum dots, Spintronics
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences > Dept of Physics and Astronomy
URI: https://discovery.ucl.ac.uk/id/eprint/10084463
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