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Virtual unrolling of spirally-wound lithium-ion cells for correlative degradation studies and predictive fault detection

Kok, MDR; Robinson, JB; Weaving, JS; Jnawali, A; Pham, M; Iacoviello, F; Brett, DJL; (2019) Virtual unrolling of spirally-wound lithium-ion cells for correlative degradation studies and predictive fault detection. Sustainable Energy & Fuels , 3 (11) pp. 2972-2976. 10.1039/c9se00500e. Green open access

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Abstract

A spirally-wound LG 18650 MJ1 lithium-ion battery was imaged in 3D before and after 1061 cycles using X-ray computed tomography. The battery's capacity had faded to 79% of its initial value and some of that fade was attributed to delamination in the innermost region of the ‘jelly-roll’ structure. A method for virtually unrolling the jelly-roll and analysing it in different coordinates is presented. The method allows efficient comparison of the position and shape of the electrodes at different times and highlights imperfections present in the jelly-roll before cycling which were shown to nucleate the delamination of the electrode.

Type: Article
Title: Virtual unrolling of spirally-wound lithium-ion cells for correlative degradation studies and predictive fault detection
Open access status: An open access version is available from UCL Discovery
DOI: 10.1039/c9se00500e
Publisher version: https://doi.org/10.1002/1873-3468.1312510.1039/c9s...
Language: English
Additional information: © The Royal Society of Chemistry 2019. This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence (http://creativecommons.org/licenses/by-nc/3.0/).
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science > Dept of Chemical Engineering
URI: https://discovery.ucl.ac.uk/id/eprint/10080515
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