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Perovskite Solar Cells with ZnO Electron-Transporting Materials

Zhang, P; Wu, J; Zhang, T; Wang, Y; Liu, D; Chen, H; Ji, L; ... Li, S; + view all (2017) Perovskite Solar Cells with ZnO Electron-Transporting Materials. Advanced Materials , 30 (3) , Article 1703737. 10.1002/adma.201703737. Green open access

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Abstract

Perovskite solar cells (PSCs) have developed rapidly over the past few years, and the power conversion efficiency of PSCs has exceeded 20%. Such high performance can be attributed to the unique properties of perovskite materials, such as high absorption over the visible range and long diffusion length. Due to the different diffusion lengths of holes and electrons, electron transporting materials (ETMs) used in PSCs play a critical role in PSCs performance. As an alternative to TiO2 ETM, ZnO materials have similar physical properties to TiO2 but with much higher electron mobility. In addition, there are many simple and facile methods to fabricate ZnO nanomaterials with low cost and energy consumption. This review focuses on recent developments in the use of ZnO ETM for PSCs. The fabrication methods of ZnO materials are briefly introduced. The influence of different ZnO ETMs on performance of PSCs is then reviewed. The limitations of ZnO ETM‐based PSCs and some solutions to these challenges are also discussed. The review provides a systematic and comprehensive understanding of the influence of different ZnO ETMs on PSCs performance and potentially motivates further development of PSCs by extending the knowledge of ZnO‐based PSCs to TiO2‐based PSCs.

Type: Article
Title: Perovskite Solar Cells with ZnO Electron-Transporting Materials
Open access status: An open access version is available from UCL Discovery
DOI: 10.1002/adma.201703737
Publisher version: https://doi.org/10.1002/adma.201703737
Language: English
Additional information: This version is the author accepted manuscript. For information on re-use, please refer to the publisher’s terms and conditions.
Keywords: Science & Technology, Physical Sciences, Technology, Chemistry, Multidisciplinary, Chemistry, Physical, Nanoscience & Nanotechnology, Materials Science, Multidisciplinary, Physics, Applied, Physics, Condensed Matter, Chemistry, Science & Technology - Other Topics, Materials Science, Physics, electron transport materials, nanostructures, perovskite solar cells, photovoltaics, zinc oxide, DOPED ZINC-OXIDE, ORGANOMETAL HALIDE PEROVSKITES, POWER CONVERSION EFFICIENCY, METHYLAMMONIUM LEAD IODIDE, THIN-FILM, OPTICAL-PROPERTIES, LOW-TEMPERATURE, SEED LAYER, INTERFACIAL MODIFICATION, SELECTIVE CONTACT
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science
URI: https://discovery.ucl.ac.uk/id/eprint/10051643
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