eprintid: 1529996 rev_number: 25 eprint_status: archive userid: 608 dir: disk0/01/52/99/96 datestamp: 2017-05-12 12:04:32 lastmod: 2021-09-25 23:02:52 status_changed: 2017-05-12 12:04:32 type: article metadata_visibility: show creators_name: Profijt, HB creators_name: Potts, SE creators_name: Van De Sanden, MCM creators_name: Kessels, WMM title: Plasma-assisted atomic layer deposition: Basics, opportunities, and challenges ispublished: pub divisions: UCL divisions: B04 divisions: C06 divisions: F56 note: This version is the version of record. For information on re-use, please refer to the publisher’s terms and conditions. abstract: Plasma-assisted atomic layer deposition (ALD) is an energy-enhanced method for the synthesis of ultra-thin films with -level resolution in which a plasma is employed during one step of the cyclic deposition process. The use of plasma species as reactants allows for more freedom in processing conditions and for a wider range of material properties compared with the conventional thermally-driven ALD method. Due to the continuous miniaturization in the microelectronics industry and the increasing relevance of ultra-thin films in many other applications, the deposition method has rapidly gained popularity in recent years, as is apparent from the increased number of articles published on the topic and plasma-assisted ALD reactors installed. To address the main differences between plasma-assisted ALD and thermal ALD, some basic aspects related to processing plasmas are presented in this review article. The plasma species and their role in the surface chemistry are addressed and different equipment configurations, including radical-enhanced ALD, direct plasma ALD, and remote plasma ALD, are described. The benefits and challenges provided by the use of a plasma step are presented and it is shown that the use of a plasma leads to a wider choice in material properties, substrate temperature, choice of precursors, and processing conditions, but that the processing can also be compromised by reduced film conformality and plasma damage. Finally, several reported emerging applications of plasma-assisted ALD are reviewed. It is expected that the merits offered by plasma-assisted ALD will further increase the interest of equipment manufacturers for developing industrial-scale deposition configurations such that the method will find its use in several manufacturing applications. © 2011 American Vacuum Society. date: 2011-09 date_type: published official_url: http://doi.org/10.1116/1.3609974 oa_status: green full_text_type: pub language: eng primo: open primo_central: open_green verified: verified_manual elements_id: 1193578 doi: 10.1116/1.3609974 lyricists_name: Potts, Stephen lyricists_id: SEPOT20 actors_name: Waragoda Vitharana, Nimal actors_id: NWARR44 actors_role: owner full_text_status: public publication: Journal of Vacuum Science and Technology A: Vacuum, Surfaces and Films volume: 29 number: 5 issn: 0734-2101 citation: Profijt, HB; Potts, SE; Van De Sanden, MCM; Kessels, WMM; (2011) Plasma-assisted atomic layer deposition: Basics, opportunities, and challenges. Journal of Vacuum Science and Technology A: Vacuum, Surfaces and Films , 29 (5) 10.1116/1.3609974 <https://doi.org/10.1116/1.3609974>. Green open access document_url: https://discovery.ucl.ac.uk/id/eprint/1529996/1/Potts_1%252E3609974.pdf