TY - JOUR A1 - Kuttatheyil, AV A1 - Laessig, D A1 - Lincke, J A1 - Kobalz, M A1 - Baias, M A1 - Koenig, K A1 - Hofmann, J A1 - Krautscheid, H A1 - Pickard, CJ A1 - Haase, J A1 - Bertmer, M JF - Inorganic Chemistry SP - 4431 N1 - This document is the Accepted Manuscript version of a Published Work that appeared in final form in Inorganic Chemistry, © 2013 American Chemical Society, after peer review and technical editing by the publisher. To access the final edited and published work see http://dx.doi.org/10.1021/ic302643w VL - 52 EP - 4442 UR - http://dx.doi.org/10.1021/ic302643w ID - discovery1396211 IS - 8 N2 - Synthesis and solid-state NMR characterization of two isomorphous series of zinc and cobalt coordination networks with 1,2,4-triazolyl benzoate ligands are reported. Both series consist of 3D diamondoid networks with four-fold interpenetration. Solid-state NMR identifies the metal coordination of the ligands, and assignment of all 1H and 13C shifts was enabled by the combination of 13C editing, FSLG-HETCOR spectra, and 2D 1H?1H back-to-back (BABA) spectra with results from NMR-CASTEP calculations. The incorporation of Co2+ replacing Zn2+ ions in the MOF over the full range of concentrations has significant influences on the NMR spectra. A uniform distribution of metal ions is documented based on the analysis of 1H T1 relaxation time measurements. AV - public TI - Synthesis, Crystal Structure, and Solid-State NMR Investigations of Heteronuclear Zn/Co Coordination Networks - A Comparative Study SN - 0020-1669 Y1 - 2013/04/15/ ER -