eprintid: 124331 rev_number: 34 eprint_status: archive userid: 608 dir: disk0/00/12/43/31 datestamp: 2010-10-23 19:30:11 lastmod: 2020-05-17 04:41:28 status_changed: 2010-10-23 19:30:11 type: article metadata_visibility: show item_issues_count: 0 creators_name: Itoh, N creators_name: Stoneham, D creators_name: Stoneham, AM title: The predose effect in thermoluminescent dosimetry ispublished: pub subjects: 11050 divisions: UCL divisions: A01 divisions: B04 divisions: C06 keywords: OPTICALLY STIMULATED LUMINESCENCE, RADIATION-INDUCED CONDUCTIVITY, SINGLE IRRADIATION EXCITATION, CRYSTALLINE SIO2, QUARTZ CRYSTALS, ELECTRODIFFUSED QUARTZ, <SIO4/LI>0 CENTER, NATURAL QUARTZ, POINT-DEFECTS, PEAK note: Text made available to UCL Discovery by kind permission of IOP Publishing, 2012 abstract: We present a model of the predose effect of thermoluminescence in crystalline quartz in terms of known impurities and defect processes. It involves the recombination-induced dissociation of an aluminium-alkali complex [Al M+] and the reaction of an alkali [M+] with an activator [X], possibly Ge, to make the former an efficient electron trap [XM+]. This excitation-induced ionic process is a new feature, in addition to the simple carrier redistribution processes usually assumed, and is consistent with a number of experiments. The test dose detects [X M+], which is present in a concentration within the dynamic range of thermoluminescence measurements. Our model enables us to understand the enhanced sensitivity of the predose method, which has been widely used in archaeological and accident dosimetry, and to link it to established impurity and defect centres in alpha -quartz. date: 2001-03-12 publisher: IOP PUBLISHING LTD official_url: http://dx.doi.org/10.1088/0953-8984/13/10/314 vfaculties: VMPS oa_status: green language: eng primo: open primo_central: open_green article_type_text: Article verified: verified_manual doi: 10.1088/0953-8984/13/10/314 language_elements: EN lyricists_name: STONEHAM, ARTHUR lyricists_id: AMSTO63 full_text_status: public publication: J PHYS-CONDENS MAT volume: 13 number: 10 pagerange: 2201 - 2209 issn: 0953-8984 citation: Itoh, N; Stoneham, D; Stoneham, AM; (2001) The predose effect in thermoluminescent dosimetry. J PHYS-CONDENS MAT , 13 (10) 2201 - 2209. 10.1088/0953-8984/13/10/314 <https://doi.org/10.1088/0953-8984%2F13%2F10%2F314>. Green open access document_url: https://discovery.ucl.ac.uk/id/eprint/124331/1/0953-8984_13_10_314.pdf