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<https://discovery.ucl.ac.uk/id/eprint/10199840> <http://purl.org/dc/terms/title> "Pore-scale study of CO2 desublimation and sublimation in a packed bed during cryogenic carbon capture"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/eprint/10199840> <http://purl.org/ontology/bibo/abstract> "Cryogenic carbon capture (CCC) is an innovative technology to desublimate CO2 out of industrial flue gases. A comprehensive understanding of CO2 desublimation and sublimation is essential for widespread application of CCC, which is highly challenging due to the complex physics behind. In this work, a lattice Boltzmann (LB) model is proposed to study CO2 desublimation and sublimation for different operating conditions, including the bed temperature (subcooling degree ∆Ts), gas feed rate (Péclet number Pe) and bed porosity (ψ). The CO2 desublimation and sublimation properties are reproduced. Interactions between convective CO2 supply and desublimation/sublimation intensity are analysed. In the single-grain case, Pe is suggested to exceed a critical value Pec at each ∆Ts to avoid the convection-limited regime. Beyond Pec, the CO2 capture rate (vc) grows monotonically with ∆Ts, indicating a desublimation-limited regime. In the packed bed case, multiple grains render the convective CO2 supply insufficient and make CCC operate under the convection-limited mechanism. Besides, in small-∆Ts and high-Pe tests, CO2 desublimation becomes insufficient compared with convective CO2 supply, thus introducing the desublimation-limited regime with severe CO2 capture capacity loss (ηd). Moreover, large ψ enhances gas mobility while decreasing cold grain volume. A moderate porosity ψc is recommended for improving the CO2 capture performance. By analysing vc and ηd, regime diagrams are proposed in ∆Ts–Pe space to show distributions of convection-limited and desublimation-limited regimes, thus suggesting optimal conditions for efficient CO2 capture. This work develops a viable LB model to examine CCC under extensive operating conditions, contributing to facilitating its application."^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/eprint/10199840> <http://purl.org/dc/terms/date> "2024-07-10" .
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