<> <http://www.w3.org/2000/01/rdf-schema#comment> "The repository administrator has not yet configured an RDF license."^^<http://www.w3.org/2001/XMLSchema#string> .
<> <http://xmlns.com/foaf/0.1/primaryTopic> <https://discovery.ucl.ac.uk/id/eprint/10194590> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://purl.org/ontology/bibo/AcademicArticle> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://purl.org/ontology/bibo/Article> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/dc/terms/title> "Chemical Conversions within the Mo–Ga–C System: Layered Solids with Variable Ga Content"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/ontology/bibo/abstract> "Layered carbides are fascinating compounds due to their enormous structural and chemical diversity, as well as their potential to possess useful and tunable functional properties. Their preparation, however, is challenging and forces synthesis scientists to develop creative and innovative strategies to access high-quality materials. One unique compound among carbides is Mo₂Ga₂C. Its structure is related to the large and steadily growing family of 211 MAX phases that crystallize in a hexagonal structure (space group P6₃/mmc) with alternating layers of edge-sharing M₆X octahedra and layers of the A-element. Mo₂Ga₂C also crystallizes in the same space group, with the difference that the A-element layer is occupied by two A-elements, here Ga, that sit right on top of each other (hence named “221” compound). Here, we propose that the Ga content in this compound is variable between 2:2, 2:1, and 2: ≤1 (and 2:0) Mo/Ga ratios. We demonstrate that one Ga layer can be selectively removed from Mo₂Ga₂C without jeopardizing the hexagonal P6₃/mmc structure. This is realized by chemical treatment of the 221 phase Mo₂Ga₂C with a Lewis acid, leading to the “conventional” 211 MAX phase Mo₂GaC. Upon further reaction with CuCl₂, more Ga is removed and replaced with Cu (instead of fully exfoliating into the Ga-free Mo₂CTx MXene), leading to Mo₂Ga₁₋ₓCuₓC still crystallizing with space group P6₃/mmc, however, with a significantly larger c-lattice parameter. Furthermore, 211 Mo₂GaC can be reacted with Ga to recover the initial 221 Mo₂Ga₂C. All three reaction pathways have not been reported previously and are supported by powder X-ray diffraction (PXRD), electron microscopy, X-ray spectroscopy, and density functional theory (DFT) calculations."^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/dc/terms/date> "2024-04-29" .
<https://discovery.ucl.ac.uk/id/document/1755945> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://purl.org/ontology/bibo/Document> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/ontology/bibo/volume> "63" .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/ontology/bibo/issue> "17" .
<https://discovery.ucl.ac.uk/id/org/ext-4c61c2a60859e59ad13248da385541e4> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Organization> .
<https://discovery.ucl.ac.uk/id/org/ext-4c61c2a60859e59ad13248da385541e4> <http://xmlns.com/foaf/0.1/name> "RSC"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/dc/terms/publisher> <https://discovery.ucl.ac.uk/id/org/ext-4c61c2a60859e59ad13248da385541e4> .
<https://discovery.ucl.ac.uk/id/publication/ext-20521553> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://purl.org/ontology/bibo/Collection> .
<https://discovery.ucl.ac.uk/id/publication/ext-20521553> <http://xmlns.com/foaf/0.1/name> "Inorganic Chemistry"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/dc/terms/isPartOf> <https://discovery.ucl.ac.uk/id/publication/ext-20521553> .
<https://discovery.ucl.ac.uk/id/publication/ext-20521553> <http://www.w3.org/2002/07/owl#sameAs> <urn:issn:20521553> .
<https://discovery.ucl.ac.uk/id/publication/ext-20521553> <http://purl.org/ontology/bibo/issn> "20521553" .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/ontology/bibo/status> <http://purl.org/ontology/bibo/status/published> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-fe042c73efcd31a3843f6e6c2632f50f> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10194590#authors> .
<https://discovery.ucl.ac.uk/id/eprint/10194590#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_1> <https://discovery.ucl.ac.uk/id/person/ext-fe042c73efcd31a3843f6e6c2632f50f> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-755e0a42f6920890620a0b6ac49417db> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10194590#authors> .
<https://discovery.ucl.ac.uk/id/eprint/10194590#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_2> <https://discovery.ucl.ac.uk/id/person/ext-755e0a42f6920890620a0b6ac49417db> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-d47ef70caaa924dfc29f1402339e6b19> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10194590#authors> .
<https://discovery.ucl.ac.uk/id/eprint/10194590#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_3> <https://discovery.ucl.ac.uk/id/person/ext-d47ef70caaa924dfc29f1402339e6b19> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-c8ffadeefd8f8d76bc48a497841afe58> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10194590#authors> .
<https://discovery.ucl.ac.uk/id/eprint/10194590#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_4> <https://discovery.ucl.ac.uk/id/person/ext-c8ffadeefd8f8d76bc48a497841afe58> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-75e5019f79e75be7fa20cec6b74d3fcd> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10194590#authors> .
<https://discovery.ucl.ac.uk/id/eprint/10194590#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_5> <https://discovery.ucl.ac.uk/id/person/ext-75e5019f79e75be7fa20cec6b74d3fcd> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-90a0258c7ca22a9bd5713283439b9d31> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10194590#authors> .
<https://discovery.ucl.ac.uk/id/eprint/10194590#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_6> <https://discovery.ucl.ac.uk/id/person/ext-90a0258c7ca22a9bd5713283439b9d31> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-3224f85254be4154e47a9667a7fe0fa4> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10194590#authors> .
<https://discovery.ucl.ac.uk/id/eprint/10194590#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_7> <https://discovery.ucl.ac.uk/id/person/ext-3224f85254be4154e47a9667a7fe0fa4> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-578172a4809e7b28452bf04f630f9b43> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10194590#authors> .
<https://discovery.ucl.ac.uk/id/eprint/10194590#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_8> <https://discovery.ucl.ac.uk/id/person/ext-578172a4809e7b28452bf04f630f9b43> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-2214358efa7578265d5f594703a2e018> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10194590#authors> .
<https://discovery.ucl.ac.uk/id/eprint/10194590#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_9> <https://discovery.ucl.ac.uk/id/person/ext-2214358efa7578265d5f594703a2e018> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-5e21ebbd38047cc6ead33792e16acac9> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10194590#authors> .
<https://discovery.ucl.ac.uk/id/eprint/10194590#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_10> <https://discovery.ucl.ac.uk/id/person/ext-5e21ebbd38047cc6ead33792e16acac9> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-1310d664c63c2ec4628be0370158d399> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10194590#authors> .
<https://discovery.ucl.ac.uk/id/eprint/10194590#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_11> <https://discovery.ucl.ac.uk/id/person/ext-1310d664c63c2ec4628be0370158d399> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-0305e1b9d857b8ad15a7d54d401ea5f9> .
<https://discovery.ucl.ac.uk/id/eprint/10194590> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10194590#authors> .
<https://discovery.ucl.ac.uk/id/eprint/10194590#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_12> <https://discovery.ucl.ac.uk/id/person/ext-0305e1b9d857b8ad15a7d54d401ea5f9> .
<https://discovery.ucl.ac.uk/id/person/ext-d47ef70caaa924dfc29f1402339e6b19> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-d47ef70caaa924dfc29f1402339e6b19> <http://xmlns.com/foaf/0.1/givenName> "Ali M"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-d47ef70caaa924dfc29f1402339e6b19> <http://xmlns.com/foaf/0.1/familyName> "Malik"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-d47ef70caaa924dfc29f1402339e6b19> <http://xmlns.com/foaf/0.1/name> "Ali M Malik"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-0305e1b9d857b8ad15a7d54d401ea5f9> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-0305e1b9d857b8ad15a7d54d401ea5f9> <http://xmlns.com/foaf/0.1/givenName> "Christina S"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-0305e1b9d857b8ad15a7d54d401ea5f9> <http://xmlns.com/foaf/0.1/familyName> "Birkel"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-0305e1b9d857b8ad15a7d54d401ea5f9> <http://xmlns.com/foaf/0.1/name> "Christina S Birkel"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-fe042c73efcd31a3843f6e6c2632f50f> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-fe042c73efcd31a3843f6e6c2632f50f> <http://xmlns.com/foaf/0.1/givenName> "Carina"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-fe042c73efcd31a3843f6e6c2632f50f> <http://xmlns.com/foaf/0.1/familyName> "Büchner"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-fe042c73efcd31a3843f6e6c2632f50f> <http://xmlns.com/foaf/0.1/name> "Carina Büchner"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-5e21ebbd38047cc6ead33792e16acac9> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-5e21ebbd38047cc6ead33792e16acac9> <http://xmlns.com/foaf/0.1/givenName> "Anna"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-5e21ebbd38047cc6ead33792e16acac9> <http://xmlns.com/foaf/0.1/familyName> "Regoutz"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-5e21ebbd38047cc6ead33792e16acac9> <http://xmlns.com/foaf/0.1/name> "Anna Regoutz"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-90a0258c7ca22a9bd5713283439b9d31> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-90a0258c7ca22a9bd5713283439b9d31> <http://xmlns.com/foaf/0.1/givenName> "Yujiang"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-90a0258c7ca22a9bd5713283439b9d31> <http://xmlns.com/foaf/0.1/familyName> "Zhu"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-90a0258c7ca22a9bd5713283439b9d31> <http://xmlns.com/foaf/0.1/name> "Yujiang Zhu"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-578172a4809e7b28452bf04f630f9b43> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-578172a4809e7b28452bf04f630f9b43> <http://xmlns.com/foaf/0.1/givenName> "Martha R"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-578172a4809e7b28452bf04f630f9b43> <http://xmlns.com/foaf/0.1/familyName> "McCartney"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-578172a4809e7b28452bf04f630f9b43> <http://xmlns.com/foaf/0.1/name> "Martha R McCartney"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-c8ffadeefd8f8d76bc48a497841afe58> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-c8ffadeefd8f8d76bc48a497841afe58> <http://xmlns.com/foaf/0.1/givenName> "John"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-c8ffadeefd8f8d76bc48a497841afe58> <http://xmlns.com/foaf/0.1/familyName> "Jamboretz"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-c8ffadeefd8f8d76bc48a497841afe58> <http://xmlns.com/foaf/0.1/name> "John Jamboretz"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-3224f85254be4154e47a9667a7fe0fa4> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-3224f85254be4154e47a9667a7fe0fa4> <http://xmlns.com/foaf/0.1/givenName> "Christoph"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-3224f85254be4154e47a9667a7fe0fa4> <http://xmlns.com/foaf/0.1/familyName> "Schlueter"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-3224f85254be4154e47a9667a7fe0fa4> <http://xmlns.com/foaf/0.1/name> "Christoph Schlueter"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-75e5019f79e75be7fa20cec6b74d3fcd> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-75e5019f79e75be7fa20cec6b74d3fcd> <http://xmlns.com/foaf/0.1/givenName> "Aysha A"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-75e5019f79e75be7fa20cec6b74d3fcd> <http://xmlns.com/foaf/0.1/familyName> "Riaz"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-75e5019f79e75be7fa20cec6b74d3fcd> <http://xmlns.com/foaf/0.1/name> "Aysha A Riaz"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-2214358efa7578265d5f594703a2e018> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-2214358efa7578265d5f594703a2e018> <http://xmlns.com/foaf/0.1/givenName> "David J"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-2214358efa7578265d5f594703a2e018> <http://xmlns.com/foaf/0.1/familyName> "Smith"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-2214358efa7578265d5f594703a2e018> <http://xmlns.com/foaf/0.1/name> "David J Smith"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-755e0a42f6920890620a0b6ac49417db> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-755e0a42f6920890620a0b6ac49417db> <http://xmlns.com/foaf/0.1/givenName> "Niels"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-755e0a42f6920890620a0b6ac49417db> <http://xmlns.com/foaf/0.1/familyName> "Kubitza"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-755e0a42f6920890620a0b6ac49417db> <http://xmlns.com/foaf/0.1/name> "Niels Kubitza"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-1310d664c63c2ec4628be0370158d399> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-1310d664c63c2ec4628be0370158d399> <http://xmlns.com/foaf/0.1/givenName> "Jochen"^^<http://www.w3.org/2001/XMLSchema#string> .
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