<> <http://www.w3.org/2000/01/rdf-schema#comment> "The repository administrator has not yet configured an RDF license."^^<http://www.w3.org/2001/XMLSchema#string> . <> <http://xmlns.com/foaf/0.1/primaryTopic> <https://discovery.ucl.ac.uk/id/eprint/10193493> . <https://discovery.ucl.ac.uk/id/eprint/10193493> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://purl.org/ontology/bibo/AcademicArticle> . <https://discovery.ucl.ac.uk/id/eprint/10193493> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://purl.org/ontology/bibo/Article> . <https://discovery.ucl.ac.uk/id/eprint/10193493> <http://purl.org/dc/terms/title> "An Alternative Cascade for the Selective Methylation of Catechols and Tetrahydroisoquinolines by O-Methyltransferases"^^<http://www.w3.org/2001/XMLSchema#string> . <https://discovery.ucl.ac.uk/id/eprint/10193493> <http://purl.org/ontology/bibo/abstract> "Methyltransferases are gaining traction as a method to achieve greener and regioselective methylations of a wide array of substrates. In this work, a halide methyltransferase biomethylation cascade was successfully adapted with the incorporation of a methionine adenosyltransferase to generate the Sâ€adenosylâ€Lâ€methionine (SAM) methylation cofactor in situ from less costly ATP and Lâ€methionine, instead of directly adding SAM to start the cascade. Furthermore, this cascade was applied to achieve novel catechol and tetrahydroisoquinoline methylations with the Oâ€methyltransferases RnCOMT, MxSafC and NpN4OMT with high conversions and regioselectivities. In addition, the cascade was successfully trialled with the less toxic methyl group donor, methyl tosylate."^^<http://www.w3.org/2001/XMLSchema#string> . <https://discovery.ucl.ac.uk/id/eprint/10193493> <http://purl.org/dc/terms/date> "2024-09-09" . <https://discovery.ucl.ac.uk/id/document/1795863> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://purl.org/ontology/bibo/Document> . <https://discovery.ucl.ac.uk/id/eprint/10193493> <http://purl.org/ontology/bibo/volume> "16" . <https://discovery.ucl.ac.uk/id/eprint/10193493> <http://purl.org/ontology/bibo/issue> "7" . <https://discovery.ucl.ac.uk/id/org/ext-e7795bc59c66fd1972aa29b4459edb20> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Organization> . <https://discovery.ucl.ac.uk/id/org/ext-e7795bc59c66fd1972aa29b4459edb20> <http://xmlns.com/foaf/0.1/name> "Wiley"^^<http://www.w3.org/2001/XMLSchema#string> . <https://discovery.ucl.ac.uk/id/eprint/10193493> <http://purl.org/dc/terms/publisher> 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<https://discovery.ucl.ac.uk/id/eprint/10193493#authors> . <https://discovery.ucl.ac.uk/id/eprint/10193493#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_3> <https://discovery.ucl.ac.uk/id/person/ext-2231ac80298466adfe821d469ff9e97b> . <https://discovery.ucl.ac.uk/id/eprint/10193493> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-bef045c94f11c40712d643e6831cfb36> . <https://discovery.ucl.ac.uk/id/eprint/10193493> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10193493#authors> . <https://discovery.ucl.ac.uk/id/eprint/10193493#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_4> <https://discovery.ucl.ac.uk/id/person/ext-bef045c94f11c40712d643e6831cfb36> . <https://discovery.ucl.ac.uk/id/eprint/10193493> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-984f7ede4b72b6021e3ab45bc8eed858> . <https://discovery.ucl.ac.uk/id/eprint/10193493> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10193493#authors> . <https://discovery.ucl.ac.uk/id/eprint/10193493#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_5> <https://discovery.ucl.ac.uk/id/person/ext-984f7ede4b72b6021e3ab45bc8eed858> . <https://discovery.ucl.ac.uk/id/eprint/10193493> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-972d2547c4a8331fb7957f2ffb4f292c> . <https://discovery.ucl.ac.uk/id/eprint/10193493> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10193493#authors> . <https://discovery.ucl.ac.uk/id/eprint/10193493#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_6> <https://discovery.ucl.ac.uk/id/person/ext-972d2547c4a8331fb7957f2ffb4f292c> . <https://discovery.ucl.ac.uk/id/eprint/10193493> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-250f7c48a0a4c55670ea7a1dcd56c1cc> . <https://discovery.ucl.ac.uk/id/eprint/10193493> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10193493#authors> . <https://discovery.ucl.ac.uk/id/eprint/10193493#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_7> <https://discovery.ucl.ac.uk/id/person/ext-250f7c48a0a4c55670ea7a1dcd56c1cc> . <https://discovery.ucl.ac.uk/id/person/ext-c25f6b8a81d1c181d9a85215e4b331ac> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> . <https://discovery.ucl.ac.uk/id/person/ext-c25f6b8a81d1c181d9a85215e4b331ac> <http://xmlns.com/foaf/0.1/givenName> "Matthew T"^^<http://www.w3.org/2001/XMLSchema#string> . <https://discovery.ucl.ac.uk/id/person/ext-c25f6b8a81d1c181d9a85215e4b331ac> <http://xmlns.com/foaf/0.1/familyName> "Salinger"^^<http://www.w3.org/2001/XMLSchema#string> . <https://discovery.ucl.ac.uk/id/person/ext-c25f6b8a81d1c181d9a85215e4b331ac> <http://xmlns.com/foaf/0.1/name> "Matthew T Salinger"^^<http://www.w3.org/2001/XMLSchema#string> . <https://discovery.ucl.ac.uk/id/person/ext-250f7c48a0a4c55670ea7a1dcd56c1cc> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> . <https://discovery.ucl.ac.uk/id/person/ext-250f7c48a0a4c55670ea7a1dcd56c1cc> <http://xmlns.com/foaf/0.1/givenName> "Helen C"^^<http://www.w3.org/2001/XMLSchema#string> . <https://discovery.ucl.ac.uk/id/person/ext-250f7c48a0a4c55670ea7a1dcd56c1cc> <http://xmlns.com/foaf/0.1/familyName> "Hailes"^^<http://www.w3.org/2001/XMLSchema#string> . <https://discovery.ucl.ac.uk/id/person/ext-250f7c48a0a4c55670ea7a1dcd56c1cc> <http://xmlns.com/foaf/0.1/name> "Helen C Hailes"^^<http://www.w3.org/2001/XMLSchema#string> . <https://discovery.ucl.ac.uk/id/person/ext-972d2547c4a8331fb7957f2ffb4f292c> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> . <https://discovery.ucl.ac.uk/id/person/ext-972d2547c4a8331fb7957f2ffb4f292c> <http://xmlns.com/foaf/0.1/givenName> "Jack WE"^^<http://www.w3.org/2001/XMLSchema#string> . <https://discovery.ucl.ac.uk/id/person/ext-972d2547c4a8331fb7957f2ffb4f292c> <http://xmlns.com/foaf/0.1/familyName> "Jeffries"^^<http://www.w3.org/2001/XMLSchema#string> . <https://discovery.ucl.ac.uk/id/person/ext-972d2547c4a8331fb7957f2ffb4f292c> <http://xmlns.com/foaf/0.1/name> "Jack WE Jeffries"^^<http://www.w3.org/2001/XMLSchema#string> . <https://discovery.ucl.ac.uk/id/person/ext-8b69fc2b33b31342830d7c304d2368e5> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> . <https://discovery.ucl.ac.uk/id/person/ext-8b69fc2b33b31342830d7c304d2368e5> <http://xmlns.com/foaf/0.1/givenName> "Daniel"^^<http://www.w3.org/2001/XMLSchema#string> . <https://discovery.ucl.ac.uk/id/person/ext-8b69fc2b33b31342830d7c304d2368e5> <http://xmlns.com/foaf/0.1/familyName> "Castellano Garrido"^^<http://www.w3.org/2001/XMLSchema#string> . <https://discovery.ucl.ac.uk/id/person/ext-8b69fc2b33b31342830d7c304d2368e5> <http://xmlns.com/foaf/0.1/name> "Daniel Castellano Garrido"^^<http://www.w3.org/2001/XMLSchema#string> . <https://discovery.ucl.ac.uk/id/person/ext-984f7ede4b72b6021e3ab45bc8eed858> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> . <https://discovery.ucl.ac.uk/id/person/ext-984f7ede4b72b6021e3ab45bc8eed858> <http://xmlns.com/foaf/0.1/givenName> "Thomas S"^^<http://www.w3.org/2001/XMLSchema#string> . <https://discovery.ucl.ac.uk/id/person/ext-984f7ede4b72b6021e3ab45bc8eed858> <http://xmlns.com/foaf/0.1/familyName> "Moody"^^<http://www.w3.org/2001/XMLSchema#string> . <https://discovery.ucl.ac.uk/id/person/ext-984f7ede4b72b6021e3ab45bc8eed858> <http://xmlns.com/foaf/0.1/name> "Thomas S Moody"^^<http://www.w3.org/2001/XMLSchema#string> . <https://discovery.ucl.ac.uk/id/person/ext-2231ac80298466adfe821d469ff9e97b> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> . <https://discovery.ucl.ac.uk/id/person/ext-2231ac80298466adfe821d469ff9e97b> <http://xmlns.com/foaf/0.1/givenName> "Eleanor D"^^<http://www.w3.org/2001/XMLSchema#string> . <https://discovery.ucl.ac.uk/id/person/ext-2231ac80298466adfe821d469ff9e97b> <http://xmlns.com/foaf/0.1/familyName> "Lamming"^^<http://www.w3.org/2001/XMLSchema#string> . <https://discovery.ucl.ac.uk/id/person/ext-2231ac80298466adfe821d469ff9e97b> <http://xmlns.com/foaf/0.1/name> "Eleanor D Lamming"^^<http://www.w3.org/2001/XMLSchema#string> . <https://discovery.ucl.ac.uk/id/person/ext-bef045c94f11c40712d643e6831cfb36> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> . <https://discovery.ucl.ac.uk/id/person/ext-bef045c94f11c40712d643e6831cfb36> <http://xmlns.com/foaf/0.1/givenName> "John M"^^<http://www.w3.org/2001/XMLSchema#string> . <https://discovery.ucl.ac.uk/id/person/ext-bef045c94f11c40712d643e6831cfb36> <http://xmlns.com/foaf/0.1/familyName> "Ward"^^<http://www.w3.org/2001/XMLSchema#string> . <https://discovery.ucl.ac.uk/id/person/ext-bef045c94f11c40712d643e6831cfb36> <http://xmlns.com/foaf/0.1/name> "John M Ward"^^<http://www.w3.org/2001/XMLSchema#string> . <https://discovery.ucl.ac.uk/id/eprint/10193493> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://eprints.org/ontology/EPrint> . <https://discovery.ucl.ac.uk/id/eprint/10193493> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://eprints.org/ontology/ArticleEPrint> . <https://discovery.ucl.ac.uk/id/eprint/10193493> <http://purl.org/dc/terms/isPartOf> <https://discovery.ucl.ac.uk/id/repository> . <https://discovery.ucl.ac.uk/id/eprint/10193493> <http://eprints.org/ontology/hasDocument> <https://discovery.ucl.ac.uk/id/document/1795863> . <https://discovery.ucl.ac.uk/id/document/1795863> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://eprints.org/ontology/Document> . <https://discovery.ucl.ac.uk/id/document/1795863> 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