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<https://discovery.ucl.ac.uk/id/eprint/10192970> <http://purl.org/dc/terms/title> "Amphiphilic electrolyte additive as an ion-flow stabilizer enables superb zinc metal batteries"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/eprint/10192970> <http://purl.org/ontology/bibo/abstract> "Irreversible Zn plating/stripping along with interfacial degradation seriously affect the practical applications of aqueous zinc-ion batteries. Herein, 3-(hydroxy(phenyl)phosphoryl)propanoic acid (HPA) is introduced as an electrolyte additive that constructs a spherical micellar molecular network via association of amphiphilic groups and multiple coordination sites to directionally adsorb/transfer Zn2+ in aqueous electrolyte, thus serving as an ion-flow stabilizer. Moreover, the strong adsorption between HPA and the zinc surface induces the formation of an in situ organic-inorganic hybrid solid electrolyte interphase layer, which further promotes the charge transfer kinetics and suppresses interfacial parasitic reactions. As a result, an ultra-high average Zn plating/stripping efficiency of 99.91% over 2100 cycles at 4 mA cm−2 is achieved. Additionally, the symmetrical cell with HPA exhibits outstanding reversibility at an unprecedentedly high current density of 120 mA cm−2. Surprisingly, the initial coulombic efficiency of Zn//Cu cell is 71.74% after 7-day calendar aging, which is better than a cell without HPA (42.59%). Furthermore, the Zn//MnO2 cell exhibits superior capacity retention of 80% after 1100 cycles at 2 A g−1 compared to the cell without HPA (37%). This study provides an in-depth insight into understanding the molecular network regulation of aqueous-based electrolytes, thus shedding light on a universal approach toward ultra-stable battery applications."^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/eprint/10192970> <http://purl.org/dc/terms/date> "2024-04-16" .
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<https://discovery.ucl.ac.uk/id/person/ext-2242478cf461c667a4a55084e241554b> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-2242478cf461c667a4a55084e241554b> <http://xmlns.com/foaf/0.1/givenName> "J"^^<http://www.w3.org/2001/XMLSchema#string> .
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<https://discovery.ucl.ac.uk/id/person/ext-7e7143b82bce34bb51c8a1a772f016b5> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-7e7143b82bce34bb51c8a1a772f016b5> <http://xmlns.com/foaf/0.1/givenName> "S"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-7e7143b82bce34bb51c8a1a772f016b5> <http://xmlns.com/foaf/0.1/familyName> "Deng"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-7e7143b82bce34bb51c8a1a772f016b5> <http://xmlns.com/foaf/0.1/name> "S Deng"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-ea68ddd307b84f40b3fb17a86fb9db6b> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-ea68ddd307b84f40b3fb17a86fb9db6b> <http://xmlns.com/foaf/0.1/givenName> "H"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-ea68ddd307b84f40b3fb17a86fb9db6b> <http://xmlns.com/foaf/0.1/familyName> "Tong"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-ea68ddd307b84f40b3fb17a86fb9db6b> <http://xmlns.com/foaf/0.1/name> "H Tong"^^<http://www.w3.org/2001/XMLSchema#string> .
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