<> <http://www.w3.org/2000/01/rdf-schema#comment> "The repository administrator has not yet configured an RDF license."^^<http://www.w3.org/2001/XMLSchema#string> .
<> <http://xmlns.com/foaf/0.1/primaryTopic> <https://discovery.ucl.ac.uk/id/eprint/10190358> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://purl.org/ontology/bibo/AcademicArticle> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://purl.org/ontology/bibo/Article> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/dc/terms/title> "Unraveling the Ultrafast Photochemical Dynamics of Nitrobenzene in Aqueous Solution"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/ontology/bibo/abstract> "Nitroaromatic compounds are major constituents of the brown carbon aerosol particles in the troposphere that absorb near-ultraviolet (UV) and visible solar radiation and have a profound effect on the Earth’s climate. The primary sources of brown carbon include biomass burning, forest fires, and residential burning of biofuels, and an important secondary source is photochemistry in aqueous cloud and fog droplets. Nitrobenzene is the smallest nitroaromatic molecule and a model for the photochemical behavior of larger nitroaromatic compounds. Despite the obvious importance of its droplet photochemistry to the atmospheric environment, there have not been any detailed studies of the ultrafast photochemical dynamics of nitrobenzene in aqueous solution. Here, we combine femtosecond transient absorption spectroscopy, time-resolved infrared spectroscopy, and quantum chemistry calculations to investigate the primary steps following the near-UV (λ ≥ 340 nm) photoexcitation of aqueous nitrobenzene. To understand the role of the surrounding water molecules in the photochemical dynamics of nitrobenzene, we compare the results of these investigations with analogous measurements in solutions of methanol, acetonitrile, and cyclohexane. We find that vibrational energy transfer to the aqueous environment quenches internal excitation, and therefore, unlike the gas phase, we do not observe any evidence for formation of photoproducts on timescales up to 500 ns. We also find that hydrogen bonding between nitrobenzene and surrounding water molecules slows the S1/S0 internal conversion process."^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/dc/terms/date> "2024-04-04" .
<https://discovery.ucl.ac.uk/id/document/1718753> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://purl.org/ontology/bibo/Document> .
<https://discovery.ucl.ac.uk/id/document/1718369> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://purl.org/ontology/bibo/Document> .
<https://discovery.ucl.ac.uk/id/org/ext-9b1c5880a971a08da83400605a5e8c13> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Organization> .
<https://discovery.ucl.ac.uk/id/org/ext-9b1c5880a971a08da83400605a5e8c13> <http://xmlns.com/foaf/0.1/name> "American Chemical Society (ACS)"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/dc/terms/publisher> <https://discovery.ucl.ac.uk/id/org/ext-9b1c5880a971a08da83400605a5e8c13> .
<https://discovery.ucl.ac.uk/id/publication/ext-16c298eaab8de29c85db4063ea203628> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://purl.org/ontology/bibo/Collection> .
<https://discovery.ucl.ac.uk/id/publication/ext-16c298eaab8de29c85db4063ea203628> <http://xmlns.com/foaf/0.1/name> "Journal of the American Chemical Society"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/dc/terms/isPartOf> <https://discovery.ucl.ac.uk/id/publication/ext-16c298eaab8de29c85db4063ea203628> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/ontology/bibo/status> <http://purl.org/ontology/bibo/status/forthcoming> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-56cfd64757cc9d44b3379134e4e0c4f4> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10190358#authors> .
<https://discovery.ucl.ac.uk/id/eprint/10190358#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_1> <https://discovery.ucl.ac.uk/id/person/ext-56cfd64757cc9d44b3379134e4e0c4f4> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-58249740d1ef7453de7d5620f2a873e5> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10190358#authors> .
<https://discovery.ucl.ac.uk/id/eprint/10190358#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_2> <https://discovery.ucl.ac.uk/id/person/ext-58249740d1ef7453de7d5620f2a873e5> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-1e3cb45b640b44d53b20fd9c037ab3a0> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10190358#authors> .
<https://discovery.ucl.ac.uk/id/eprint/10190358#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_3> <https://discovery.ucl.ac.uk/id/person/ext-1e3cb45b640b44d53b20fd9c037ab3a0> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-e09b3f5b9a0abc03ac36fd2f5aa365ca> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10190358#authors> .
<https://discovery.ucl.ac.uk/id/eprint/10190358#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_4> <https://discovery.ucl.ac.uk/id/person/ext-e09b3f5b9a0abc03ac36fd2f5aa365ca> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-44c13a6aef94643712527dd8330a4aa4> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10190358#authors> .
<https://discovery.ucl.ac.uk/id/eprint/10190358#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_5> <https://discovery.ucl.ac.uk/id/person/ext-44c13a6aef94643712527dd8330a4aa4> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-8ef76b0ff9fe31af97be0c29d6ed475e> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10190358#authors> .
<https://discovery.ucl.ac.uk/id/eprint/10190358#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_6> <https://discovery.ucl.ac.uk/id/person/ext-8ef76b0ff9fe31af97be0c29d6ed475e> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-6fe02e95836e0573f4083b0f854d8ad7> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10190358#authors> .
<https://discovery.ucl.ac.uk/id/eprint/10190358#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_7> <https://discovery.ucl.ac.uk/id/person/ext-6fe02e95836e0573f4083b0f854d8ad7> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-2014a36c74adb782af57b31c1c6bcee2> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10190358#authors> .
<https://discovery.ucl.ac.uk/id/eprint/10190358#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_8> <https://discovery.ucl.ac.uk/id/person/ext-2014a36c74adb782af57b31c1c6bcee2> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-fa842dd741af0d24beb14bc62816448f> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10190358#authors> .
<https://discovery.ucl.ac.uk/id/eprint/10190358#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_9> <https://discovery.ucl.ac.uk/id/person/ext-fa842dd741af0d24beb14bc62816448f> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-fb0c4073ae9e75156624a3156917fd71> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10190358#authors> .
<https://discovery.ucl.ac.uk/id/eprint/10190358#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_10> <https://discovery.ucl.ac.uk/id/person/ext-fb0c4073ae9e75156624a3156917fd71> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-517f1e7dec43b0555072e9c47e4346ae> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10190358#authors> .
<https://discovery.ucl.ac.uk/id/eprint/10190358#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_11> <https://discovery.ucl.ac.uk/id/person/ext-517f1e7dec43b0555072e9c47e4346ae> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-815bc9493b7153c84970e3ebdb629e97> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10190358#authors> .
<https://discovery.ucl.ac.uk/id/eprint/10190358#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_12> <https://discovery.ucl.ac.uk/id/person/ext-815bc9493b7153c84970e3ebdb629e97> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/dc/terms/creator> <https://discovery.ucl.ac.uk/id/person/ext-15b5136b089f721bc419238ac8dd3be9> .
<https://discovery.ucl.ac.uk/id/eprint/10190358> <http://purl.org/ontology/bibo/authorList> <https://discovery.ucl.ac.uk/id/eprint/10190358#authors> .
<https://discovery.ucl.ac.uk/id/eprint/10190358#authors> <http://www.w3.org/1999/02/22-rdf-syntax-ns#_13> <https://discovery.ucl.ac.uk/id/person/ext-15b5136b089f721bc419238ac8dd3be9> .
<https://discovery.ucl.ac.uk/id/person/ext-56cfd64757cc9d44b3379134e4e0c4f4> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-56cfd64757cc9d44b3379134e4e0c4f4> <http://xmlns.com/foaf/0.1/givenName> "Nicholas A"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-56cfd64757cc9d44b3379134e4e0c4f4> <http://xmlns.com/foaf/0.1/familyName> "Lau"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-56cfd64757cc9d44b3379134e4e0c4f4> <http://xmlns.com/foaf/0.1/name> "Nicholas A Lau"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-815bc9493b7153c84970e3ebdb629e97> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-815bc9493b7153c84970e3ebdb629e97> <http://xmlns.com/foaf/0.1/givenName> "Andrew J"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-815bc9493b7153c84970e3ebdb629e97> <http://xmlns.com/foaf/0.1/familyName> "Orr-Ewing"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-815bc9493b7153c84970e3ebdb629e97> <http://xmlns.com/foaf/0.1/name> "Andrew J Orr-Ewing"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-6fe02e95836e0573f4083b0f854d8ad7> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-6fe02e95836e0573f4083b0f854d8ad7> <http://xmlns.com/foaf/0.1/givenName> "Julia A"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-6fe02e95836e0573f4083b0f854d8ad7> <http://xmlns.com/foaf/0.1/familyName> "Davies"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-6fe02e95836e0573f4083b0f854d8ad7> <http://xmlns.com/foaf/0.1/name> "Julia A Davies"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-2014a36c74adb782af57b31c1c6bcee2> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-2014a36c74adb782af57b31c1c6bcee2> <http://xmlns.com/foaf/0.1/givenName> "Gabriel"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-2014a36c74adb782af57b31c1c6bcee2> <http://xmlns.com/foaf/0.1/familyName> "Karras"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-2014a36c74adb782af57b31c1c6bcee2> <http://xmlns.com/foaf/0.1/name> "Gabriel Karras"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-1e3cb45b640b44d53b20fd9c037ab3a0> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-1e3cb45b640b44d53b20fd9c037ab3a0> <http://xmlns.com/foaf/0.1/givenName> "Susannah"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-1e3cb45b640b44d53b20fd9c037ab3a0> <http://xmlns.com/foaf/0.1/familyName> "Bourne-Worster"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-1e3cb45b640b44d53b20fd9c037ab3a0> <http://xmlns.com/foaf/0.1/name> "Susannah Bourne-Worster"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-e09b3f5b9a0abc03ac36fd2f5aa365ca> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-e09b3f5b9a0abc03ac36fd2f5aa365ca> <http://xmlns.com/foaf/0.1/givenName> "Rhea"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-e09b3f5b9a0abc03ac36fd2f5aa365ca> <http://xmlns.com/foaf/0.1/familyName> "Kumar"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-e09b3f5b9a0abc03ac36fd2f5aa365ca> <http://xmlns.com/foaf/0.1/name> "Rhea Kumar"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-15b5136b089f721bc419238ac8dd3be9> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-15b5136b089f721bc419238ac8dd3be9> <http://xmlns.com/foaf/0.1/givenName> "Helen H"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-15b5136b089f721bc419238ac8dd3be9> <http://xmlns.com/foaf/0.1/familyName> "Fielding"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-15b5136b089f721bc419238ac8dd3be9> <http://xmlns.com/foaf/0.1/name> "Helen H Fielding"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-fb0c4073ae9e75156624a3156917fd71> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-fb0c4073ae9e75156624a3156917fd71> <http://xmlns.com/foaf/0.1/givenName> "Gregory M"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-fb0c4073ae9e75156624a3156917fd71> <http://xmlns.com/foaf/0.1/familyName> "Greetham"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-fb0c4073ae9e75156624a3156917fd71> <http://xmlns.com/foaf/0.1/name> "Gregory M Greetham"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-fa842dd741af0d24beb14bc62816448f> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-fa842dd741af0d24beb14bc62816448f> <http://xmlns.com/foaf/0.1/givenName> "Ian P"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-fa842dd741af0d24beb14bc62816448f> <http://xmlns.com/foaf/0.1/familyName> "Clark"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-fa842dd741af0d24beb14bc62816448f> <http://xmlns.com/foaf/0.1/name> "Ian P Clark"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-517f1e7dec43b0555072e9c47e4346ae> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-517f1e7dec43b0555072e9c47e4346ae> <http://xmlns.com/foaf/0.1/givenName> "Graham A"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-517f1e7dec43b0555072e9c47e4346ae> <http://xmlns.com/foaf/0.1/familyName> "Worth"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-517f1e7dec43b0555072e9c47e4346ae> <http://xmlns.com/foaf/0.1/name> "Graham A Worth"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-58249740d1ef7453de7d5620f2a873e5> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-58249740d1ef7453de7d5620f2a873e5> <http://xmlns.com/foaf/0.1/givenName> "Deborin"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-58249740d1ef7453de7d5620f2a873e5> <http://xmlns.com/foaf/0.1/familyName> "Ghosh"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-58249740d1ef7453de7d5620f2a873e5> <http://xmlns.com/foaf/0.1/name> "Deborin Ghosh"^^<http://www.w3.org/2001/XMLSchema#string> .
<https://discovery.ucl.ac.uk/id/person/ext-44c13a6aef94643712527dd8330a4aa4> <http://www.w3.org/1999/02/22-rdf-syntax-ns#type> <http://xmlns.com/foaf/0.1/Person> .
<https://discovery.ucl.ac.uk/id/person/ext-44c13a6aef94643712527dd8330a4aa4> <http://xmlns.com/foaf/0.1/givenName> "William A"^^<http://www.w3.org/2001/XMLSchema#string> .
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