eprintid: 10090448 rev_number: 18 eprint_status: archive userid: 608 dir: disk0/10/09/04/48 datestamp: 2021-08-09 16:49:03 lastmod: 2021-10-21 23:21:54 status_changed: 2021-08-09 16:49:03 type: working_paper metadata_visibility: show creators_name: Pereira, P creators_name: Gustafsson, N creators_name: Marsh, M creators_name: Mhlanga, M creators_name: Henriques, R title: Super-Beacons: open-source probes with spontaneous tuneable blinking compatible with live-cell super-resolution microscopy ispublished: pub divisions: UCL divisions: B02 divisions: C08 divisions: D77 note: The copyright holder for this preprint is the author/funder, who has granted bioRxiv a license to display the preprint in perpetuity. It is made available under a CC-BY 4.0 International license (http://creativecommons.org/licenses/by/4.0/). abstract: Localization based super-resolution microscopy relies on the detection of individual molecules cycling between fluorescent and non-fluorescent states. These transitions are commonly regulated by high-intensity illumination, imposing constrains to imaging hardware and producing sample photodamage. Here, we propose single-molecule self-quenching as a mechanism to generate spontaneous photoswitching independent of illumination. To demonstrate this principle, we developed a new class of DNA-based open-source Super-Resolution probes named Super-Beacons, with photoswitching kinetics that can be tuned structurally, thermally and chemically. The potential of these probes for live-cell friendly Super-Resolution Microscopy without high-illumination or toxic imaging buffers is revealed by imaging Interferon Inducible Transmembrane proteins (IFITMs) at sub-100nm resolutions. date: 2020-02-04 publisher: BioRxiv official_url: https://doi.org/10.1101/2020.01.20.912311 oa_status: green full_text_type: pub language: eng primo: open primo_central: open_green verified: verified_manual elements_id: 1744615 doi: 10.1101/2020.01.20.912311 lyricists_name: Henriques, Ricardo Jose lyricists_name: Marsh, Mark lyricists_id: RJSDH70 lyricists_id: MCPMA80 actors_name: Henriques, Ricardo Jose actors_id: RJSDH70 actors_role: owner full_text_status: public place_of_pub: Cold Spring Harbor, NY, USA pages: 11 citation: Pereira, P; Gustafsson, N; Marsh, M; Mhlanga, M; Henriques, R; (2020) Super-Beacons: open-source probes with spontaneous tuneable blinking compatible with live-cell super-resolution microscopy. BioRxiv: Cold Spring Harbor, NY, USA. Green open access document_url: https://discovery.ucl.ac.uk/id/eprint/10090448/1/2020.01.20.912311v1.full.pdf