eprintid: 10074888 rev_number: 23 eprint_status: archive userid: 608 dir: disk0/10/07/48/88 datestamp: 2019-05-29 13:04:10 lastmod: 2021-11-23 01:16:36 status_changed: 2019-05-29 13:04:10 type: article metadata_visibility: show creators_name: Ren, Q creators_name: You, JW creators_name: Panoiu, NC title: Large enhancement of the effective second-order nonlinearity in graphene metasurfaces ispublished: pub divisions: UCL divisions: B04 divisions: C05 divisions: F46 note: This version is the version of record. For information on re-use, please refer to the publisher’s terms and conditions. abstract: Using a powerful homogenization technique, one- and two-dimensional graphene metasurfaces are homogenized both at the fundamental frequency (FF) and second harmonic (SH). In both cases, there is excellent agreement between the predictions of the homogenization method and those based on rigorous numerical solutions of Maxwell equations. The homogenization technique is then employed to demonstrate that, owing to a double-resonant plasmon excitation mechanism that leads to strong, simultaneous field enhancement at the FF and SH, the effective second-order susceptibility of graphene metasurfaces can be enhanced by more than three orders of magnitude as compared to the intrinsic second-order susceptibility of a graphene sheet placed on the same substrate. In addition, we explore the implications of our results on the development of new active nanodevices that incorporate nanopatterned graphene structures. date: 2019-05-15 date_type: published publisher: AMER PHYSICAL SOC official_url: https://doi.org/10.1103/PhysRevB.99.205404 oa_status: green full_text_type: pub language: eng primo: open primo_central: open_green verified: verified_manual elements_id: 1660013 doi: 10.1103/PhysRevB.99.205404 lyricists_name: Panoiu, Nicolae-Coriolan lyricists_name: You, Jianwei lyricists_id: NPANO59 lyricists_id: JWYOU76 actors_name: Allington-Smith, Dominic actors_id: DAALL44 actors_role: owner full_text_status: public publication: Physical Review B volume: 99 number: 20 article_number: 205404 pages: 10 issn: 2469-9969 citation: Ren, Q; You, JW; Panoiu, NC; (2019) Large enhancement of the effective second-order nonlinearity in graphene metasurfaces. Physical Review B , 99 (20) , Article 205404. 10.1103/PhysRevB.99.205404 <https://doi.org/10.1103/PhysRevB.99.205404>. Green open access document_url: https://discovery.ucl.ac.uk/id/eprint/10074888/1/Panoiu_PhysRevB.99.205404.pdf