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Enhancement of H-2 uptake via fluorination but not lithiation for Zn4N8 and Zn4N6O type clusters

Redshaw, C; Jana, S; Shang, CX; Elsegood, MRJ; Lu, XS; Guo, ZX; (2010) Enhancement of H-2 uptake via fluorination but not lithiation for Zn4N8 and Zn4N6O type clusters. CHEM COMMUN , 46 (47) 9055 - 9057. 10.1039/c0cc03380d.

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Abstract

The introduction of fluorinated aryls at zinc in Zn4N8-type (and to a lesser extent Zn4N6O) cages led to enhanced H-2 uptake. Lithium alkoxides have been shown to link such cages (non-fluorinated), but showed no substantial improvement in uptake.

Type: Article
Title: Enhancement of H-2 uptake via fluorination but not lithiation for Zn4N8 and Zn4N6O type clusters
DOI: 10.1039/c0cc03380d
Keywords: METAL-ORGANIC FRAMEWORKS, HYDROGEN ADSORPTION, GAS-ADSORPTION, ZINC ALKYLS, OXYGENATION, COMPLEX, STORAGE
UCL classification: UCL > School of BEAMS > Faculty of Maths and Physical Sciences > Chemistry
URI: http://discovery.ucl.ac.uk/id/eprint/706295
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