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Two stage fluid bed-plasma gasification process for solid waste valorisation: technical review and preliminary thermodynamic modelling of sulphur emissions.

Morrin, S; Lettieri, P; Chapman, C; Mazzei, L; (2011) Two stage fluid bed-plasma gasification process for solid waste valorisation: technical review and preliminary thermodynamic modelling of sulphur emissions. Waste Management , 32 (4) 676 - 684. 10.1016/j.wasman.2011.08.020. Green open access

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Abstract

Gasification of solid waste for energy has significant potential given an abundant feed supply and strong policy drivers. Nonetheless, significant ambiguities in the knowledge base are apparent. Consequently this study investigates sulphur mechanisms within a novel two stage fluid bed-plasma gasification process. This paper includes a detailed review of gasification and plasma fundamentals in relation to the specific process, along with insight on MSW based feedstock properties and sulphur pollutant therein. As a first step to understanding sulphur partitioning and speciation within the process, thermodynamic modelling of the fluid bed stage has been performed. Preliminary findings, supported by plant experience, indicate the prominence of solid phase sulphur species (as opposed to H(2)S) - Na and K based species in particular. Work is underway to further investigate and validate this.

Type: Article
Title: Two stage fluid bed-plasma gasification process for solid waste valorisation: technical review and preliminary thermodynamic modelling of sulphur emissions.
Location: United States
Open access status: An open access version is available from UCL Discovery
DOI: 10.1016/j.wasman.2011.08.020
Publisher version: http://dx.doi.org/10.1016/j.wasman.2011.08.020
Language: English
Additional information: This is an open-access article distributed under the terms of the Creative Commons Attribution License (CC BY), which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.
Keywords: Conservation of Natural Resources, Environmental Pollutants, Hot Temperature, Models, Chemical, Plasma Gases, Refuse Disposal, Sulfur, Thermodynamics
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science > Dept of Chemical Engineering
URI: https://discovery.ucl.ac.uk/id/eprint/1327339
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