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Growth mechanisms for InAs/GaAs QDs with and without Bi surfactants

Chen, XY; Gu, Y; Ma, YJ; Chen, SM; Tang, MC; Zhang, YY; Yu, XZ; ... Zhang, YG; + view all (2019) Growth mechanisms for InAs/GaAs QDs with and without Bi surfactants. Materials Research Express , 6 (1) 10.1088/2053-1591/aae85d. Green open access

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Abstract

We report systematic study of growth of self-assembled InAs quantum dots (QDs) on GaAs substrate at various temperatures with and without exposure of bismuth surfactants. Results show that the coalescence amongst InAs QDs is considerably inhibited by the exposure of bismuth flux during growth in the temperature range from 475 to 500 °C, leading to improved dot uniformity and a modified dot density. The mechanism of the suppression effect by bismuth surfactants on the strain-induced islanding through inhibiting the indium adatom mobility and the evaporation rate on the surface kinetically is thus clarified for the growth of InAs QDs. The photoluminescence peak wavelength for the InAs QDs with Bi exposure red shifted slightly due to the suppression of Bi atoms on the QD dissolution during the capping process at higher temperatures. Moreover, by investigating the temperature-dependent quenching processes with and without Bi exposure, it is observed that the the weak carrier confinement occurred in QDs with the presence of Bi caused broadness in the linewidths.

Type: Article
Title: Growth mechanisms for InAs/GaAs QDs with and without Bi surfactants
Open access status: An open access version is available from UCL Discovery
DOI: 10.1088/2053-1591/aae85d
Publisher version: https://doi.org/10.1088/2053-1591/aae85d
Language: English
Additional information: This version is the author accepted manuscript. For information on re-use, please refer to the publisher’s terms and conditions.
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science > Dept of Electronic and Electrical Eng
URI: https://discovery.ucl.ac.uk/id/eprint/10066158
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