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In situ compression and X-ray computed tomography of flow battery electrodes

Jervis, R; Kok, MDR; Neville, TP; Meyer, Q; Brown, LD; Iacoviello, F; Gostick, JT; ... Shearing, PR; + view all (2018) In situ compression and X-ray computed tomography of flow battery electrodes. Journal of Energy Chemistry , 27 (5) pp. 1353-1361. 10.1016/j.jechem.2018.03.022. Green open access

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Abstract

Redox flow batteries offer a potential solution to an increase in renewable energy generation on the grid by offering long-term, large-scale storage and regulation of power. However, they are currently underutilised due to cost and performance issues, many of which are linked to the microstructure of the porous carbon electrodes used. Here, for the first time, we offer a detailed study of the in situ effects of compression on a commercially available carbon felt electrode. Visualisation of electrode structure using X-ray computed tomography shows the non-linear way that these materials compress and various metrics are used to elucidate the changes in porosity, pore size distribution and tortuosity factor under compressions from 0%–90%.

Type: Article
Title: In situ compression and X-ray computed tomography of flow battery electrodes
Open access status: An open access version is available from UCL Discovery
DOI: 10.1016/j.jechem.2018.03.022
Publisher version: https://doi.org/10.1016/j.jechem.2018.03.022
Language: English
Additional information: This version is the author accepted manuscript. For information on re-use, please refer to the publisher’s terms and conditions.
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science > Dept of Chemical Engineering
URI: https://discovery.ucl.ac.uk/id/eprint/10051832
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