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Doping-induced quantum crossover in Er2Ti2-xSnxO7

Shirai, M; Freitas, RS; Lago, J; Bramwell, ST; Ritter, C; Zivkovic, I; (2017) Doping-induced quantum crossover in Er2Ti2-xSnxO7. Physical Review B , 96 , Article 180411(R). 10.1103/PhysRevB.96.180411. Green open access

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Abstract

We present the results of the investigation of magnetic properties of the Er 2 Ti 2 − x Sn x O 7 series. For small doping values, the ordering temperature decreases linearly with x , while the moment configuration remains the same as in the x = 0 parent compound. Around x = 1.7 doping level, we observe a change in the behavior, where the ordering temperature starts to increase and new magnetic Bragg peaks appear. For the first time, we present evidence of a long-range order (LRO) in Er 2 Sn 2 O 7 ( x = 2.0 ) below T N = 130 mK. It is revealed that the moment configuration corresponds to a Palmer-Chalker type with a value of the magnetic moment significantly renormalized compared to x = 0 . We discuss our results in the framework of a possible quantum phase transition occurring close to x = 1.7 .

Type: Article
Title: Doping-induced quantum crossover in Er2Ti2-xSnxO7
Open access status: An open access version is available from UCL Discovery
DOI: 10.1103/PhysRevB.96.180411
Publisher version: https://doi.org/10.1103/PhysRevB.96.180411
Language: English
Additional information: This version is the version of record. For information on re-use, please refer to the publisher’s terms and conditions.
Keywords: Science & Technology, Physical Sciences, Physics, Condensed Matter, Physics, SPIN ICE, PYROCHLORE ANTIFERROMAGNET, ORDER
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences > Dept of Physics and Astronomy
URI: https://discovery.ucl.ac.uk/id/eprint/10040955
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