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Carbon Capture from Natural Gas Combined Cycle Power Plants: Solvent Performance Comparison at an Industrial Scale

Sharifzadeh, M; Shah, N; (2016) Carbon Capture from Natural Gas Combined Cycle Power Plants: Solvent Performance Comparison at an Industrial Scale. AIChE Journal , 62 (1) pp. 166-179. 10.1002/aic.15072. Green open access

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Abstract

Natural gas is an important source of energy. This article addresses the problem of integrating an existing natural gas combined cycle (NGCC) power plant with a carbon capture process using various solvents. The power plant and capture process have mutual interactions in terms of the flue gas flow rate and composition vs. the extracted steam required for solvent regeneration. Therefore, evaluating solvent performance at a single (nominal) operating point is not indicative and solvent performance should be considered subject to the overall process operability and over a wide range of operating conditions. In the present research, a novel optimization framework was developed in which design and operation of the capture process are optimized simultaneously and their interactions with the upstream power plant are fully captured. The developed framework was applied for solvent comparison which demonstrated that GCCmax, a newly developed solvent, features superior performances compared to the monoethanolamine baseline solvent.

Type: Article
Title: Carbon Capture from Natural Gas Combined Cycle Power Plants: Solvent Performance Comparison at an Industrial Scale
Open access status: An open access version is available from UCL Discovery
DOI: 10.1002/aic.15072
Publisher version: http://dx.doi.org/10.1002/aic.15072
Language: English
Additional information: This version is the author accepted manuscript. For information on re-use, please refer to the publisher’s terms and conditions.
Keywords: Science & Technology, Technology, Engineering, Chemical, Engineering, CO2, carbon capture, natural gas combined cycle (NGCC) power plant, energy efficiency, integrated process design and control, GCCmax, POSTCOMBUSTION CO2 CAPTURE, CONTROLLED PROCESS MODEL, STRIPPER CONFIGURATIONS, INTEGRATED DESIGN, OPTIMIZATION, DISTILLATION, METHODOLOGY, OPERATION, DIOXIDE, SYSTEMS
UCL classification: UCL
UCL > Provost and Vice Provost Offices
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science
URI: https://discovery.ucl.ac.uk/id/eprint/10023923
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